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Separated Anode Experiment to Measure Gas Transport and Methane Reforming within Solid-Oxide Fuel Cell Anodes

Published online by Cambridge University Press:  22 May 2012

Amy E. Richards
Affiliation:
Mechanical Engineering, Colorado School of Mines, Golden, CO 80401, USA
Neal P. Sullivan
Affiliation:
Mechanical Engineering, Colorado School of Mines, Golden, CO 80401, USA
Huayang Zhu
Affiliation:
Mechanical Engineering, Colorado School of Mines, Golden, CO 80401, USA
Robert J. Kee
Affiliation:
Mechanical Engineering, Colorado School of Mines, Golden, CO 80401, USA
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Abstract

Solid-oxide fuel cell (SOFC) performance depends greatly upon electrode design. The composite anode plays a critical role in fuel reforming, especially when hydrocarbons are included in the fuel mixture. Because direct observation of fuel reforming in a functioning SOFC is difficult, if not impossible, an alternative experimental configuration is needed to evaluate anode performance. The Separated Anode Experiment (SAE) is designed to isolate and study porous-media transport and heterogeneous reforming chemistry in SOFC anodes. Although the experiment does not incorporate a dense electrolyte membrane or a cathode, it is configured to replicate important aspects of anode behavior in a fully operational SOFC. The experiment is also designed to facilitate model-based interpretation of the results. Comparisons of two significantly different anode structures are used to illustrate the experimental and modeling capabilities.

Type
Research Article
Copyright
Copyright © Materials Research Society 2012

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