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Modification with ultrasonication for enhanced properties of cobalt-based zeolitic imidazolate framework

Published online by Cambridge University Press:  28 August 2018

Shuyang Sun ,
Pengcheng Wang  and
Ming Lu Open the ORCID record for Ming Lu [Opens in a new window]
Shuyang Sun
Affiliation:
School of Chemical Engineering, Nanjing University of Science and Technology, Nanjing 210094, Jiangsu Province, People's Republic of China
Pengcheng Wang
Affiliation:
School of Chemical Engineering, Nanjing University of Science and Technology, Nanjing 210094, Jiangsu Province, People's Republic of China
Ming Lu*
Affiliation:
School of Chemical Engineering, Nanjing University of Science and Technology, Nanjing 210094, Jiangsu Province, People's Republic of China
*
Address all correspondence to Lu Ming at [email protected]
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Abstract

Effective modification of existing supported catalyst has attracted plenty of interests recently. Herein, we introduced ultrasonication to synthesize the palladium-loaded cobalt-based zeolitic imidazolate framework and compared its properties with those using the conventional method. Remarkably, the ultrasonicated frameworks possess 15.33% higher of Brunauer–Emmett–Teller (BET) surface area and 63.37% higher of t-plot external surface area, respectively, which lead up to 23% rise in the degradation of organic pollutants under optimized conditions. Characterizations clearly revealed the causality between ultrasonication, morphology, and catalytic performance compared with their non-ultrasonicated counterparts which further demonstrates a simple but useful method for the modification of supported catalysts.

Type
Research Letters
Information
MRS Communications , Volume 8 , Issue 3 , September 2018 , pp. 1363 - 1370
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Copyright
Copyright © Materials Research Society 2018 

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