For mobile 3-D radar installed on a gyro-stabilized platform, its measurements are usually contaminated by the systematic biases which contain radar offset biases (i.e., range, azimuth and elevation biases) and attitude biases (i.e., yaw, pitch and roll biases) of the platform because of the errors in the Inertial Measurement Units (IMU). Systematic biases can NOT be removed by a single radar itself; however, fortunately, they can be estimated by using two different radar measurements of the same target. The process of estimating systematic biases and then compensating radar measurements is called error registration. In this paper, the registration models are established first, then, the equivalent radar measurement error expressions caused by the attitude biases are derived and the dependencies among attitude biases and offset biases are analysed by using the observable matrix criterion. Based on the analyses above, an Optimized Bias Estimation Model (OBEM) is proposed for registration. OBEM uses the subtraction of azimuth and yaw bias as one variable and omits roll and pitch biases in the state vector, which decreases the dimension of the state vector from fourteen of the All Augmented Model (AAM), (which uses all the systematic biases of both radars as state vector) to eight and has about 80% reduction in calculation costs. Also, OBEM can decrease the coupling influences of roll and pitch biases and improve the estimation performance of radar elevation bias. Monte Carlo experiments were made. Numerical results showed that the bias estimation accuracies and the rectified radar raw measurement accuracies can be improved.