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Scanning probe microscopy, luminescence and third harmonic generation studies of elongated CdS:Mn nanostructures developed by energetic oxygen-ion-impact

Published online by Cambridge University Press:  06 July 2006

D. Mohanta ,
G. A. Ahmed ,
A. Choudhury ,
F. Singh ,
D. K. Avasthi ,
G. Boyer  and
G. A. Stanciu
D. Mohanta*
Affiliation:
Department of Physics, Tezpur University, PO Napaam, Assam – 784 028, India
G. A. Ahmed
Affiliation:
Department of Physics, Tezpur University, PO Napaam, Assam – 784 028, India
A. Choudhury
Affiliation:
Department of Physics, Tezpur University, PO Napaam, Assam – 784 028, India
F. Singh
Affiliation:
Inter University Accelerator Centre, Aruna Asaf Ali Marg, New Delhi – 110 067, India
D. K. Avasthi
Affiliation:
Inter University Accelerator Centre, Aruna Asaf Ali Marg, New Delhi – 110 067, India
G. Boyer
Affiliation:
Laboratoire d'Optique Appliquée, ENSTA - École polytechnique, Centre de l'Yvette, 91128 Palaiseau Cedex, France
G. A. Stanciu
Affiliation:
University “Politehnica” of Bucharest, 313 Splaiul Independentei str., sector 6, 060032 Bucharest, Romania
*
[email protected]
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Abstract

Manganese-doped cadmium sulfide nanoparticles are synthesized in a flexible polymer matrix (synthetic rubber) by a chemical route. They are bombarded with 80-MeV oxygen ions having electronic energy loss (S e ) dominant over nuclear energy loss (S n ) and with fluence variation 1011–1013 ions/cm2. Piling up of nanoparticles along certain direction was observed in atomic force microscopy (AFM) images of irradiated samples. Such elongated nanostructures are as a result of nanoparticle growth during ion passage through the samples. Specifically, elongated structures in the form of nanoneedles, nanochannels and nanorods have been observed. The fluence dependent photoluminescence spectra (PL) show significant luminescent peaks at 445 nm and 706 nm, respectively which are tunable with ion fluence. Such a tunability could be promising as lasing materials in nano-luminescent devices and laser diodes. Further, detection of efficient third harmonic generation (THG) in these samples (by using irradiation of a Cr:fosterite laser) could be promising in nanoscopy and nonlinear optics.

Keywords

Type
Research Article
Information
The European Physical Journal - Applied Physics , Volume 35 , Issue 1 , July 2006 , pp. 29 - 36
Copyright
© EDP Sciences, 2006

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