Hostname: page-component-78c5997874-t5tsf Total loading time: 0 Render date: 2024-11-20T01:38:26.420Z Has data issue: false hasContentIssue false

Radiocarbon in Seawater at Radioactive Waste Dumping Sites in the Northeast Atlantic and Northwest Pacific

Published online by Cambridge University Press:  18 July 2016

P P Povinec
Affiliation:
International Atomic Energy Agency, Marine Environmental Laboratory, 4 Quai Antoine 1er, MC-98012, Monaco. Email: [email protected].
A J T Jull
Affiliation:
The University of Arizona, NSF Arizona AMS Facility, Department of Physics, Tucson, Arizona 85721, USA
G S Burr
Affiliation:
The University of Arizona, NSF Arizona AMS Facility, Department of Physics, Tucson, Arizona 85721, USA
Rights & Permissions [Opens in a new window]

Abstract

Core share and HTML view are not available for this content. However, as you have access to this content, a full PDF is available via the ‘Save PDF’ action button.

Radiocarbon has been an important constituent of radioactive wastes dumped in the open ocean and marginal seas as well as wastes released from nuclear reprocessing plants. Therefore, in some regions these sources could have a greater impact on 14C concentration in seawater than global fallout. The high analytical sensitivity of 14C measurement by accelerator mass spectrometry (AMS) allows even tracer amounts of 14C to be found in seawater at radioactive waste dumping sites and their comparison with the global distribution of this radionuclide. Data on measurements of 14C in samples taken at former dumping sites in the northeast Atlantic and northwest Pacific Oceans and in the open ocean are discussed and compared with other anthropogenic radionuclides, namely 3H. Small increases in 14C concentrations observed in some bottom and surface seawater samples collected at the Northwest Pacific Ocean dumping sites require further 14C analyses before final conclusions can be made on possible leakages from dumped radioactive wastes.

Type
II. Our ‘Wet’ Environment
Copyright
Copyright © 2001 by the Arizona Board of Regents on behalf of the University of Arizona 

References

Aramaki, T, Mishizuma, T, Kuji, T, Povinec, PP, Togawa, O. 2000. Distribution of radiocarbon in the southwestern North Pacific. Radiocarbon. This issue.Google Scholar
Baxter, MS, Ballestra, S, Gastaud, J, Hamilton, TF, Harms, I, Huynh-Ngoc, L, Liong Wee Kwong, L, Osvath, I, Parsi, P, Pettersson, H, Povinec, PP, Sanchez, A. 1995. Marine radioactivity studies in the vicinity of sites with potential radionuclide releases. In: Environmental Impact of Radioactive Releases, Proceedings of an International Symposium on Environmental Impact of Radioactive Releases IAEA, Vienna, 8-12 May 1995. International Atomic Energy Agency, Vienna: 125142.Google Scholar
Broecker, WS. 1991. The great ocean conveyor. Oceanography 4:7989.Google Scholar
Broecker, WS, Peng, TH. 1992. Interhemispheric transport of carbon dioxide by ocean circulation. Nature 356:587589.CrossRefGoogle Scholar
Donahue, DJ, Linick, TW, Jull, AJT. 1990a. Isotope-ratio and background corrections for accelerator mass spectrometry radiocarbon measurements. Radiocarbon 32(2):135142.CrossRefGoogle Scholar
Donahue, DJ, Jull, AJT, Toolin, LJ. 1990b. Radiocarbon measurements at the University of Arizona AMS Facility. Nuclear Instruments and Methods in Physics Research B52:224228.CrossRefGoogle Scholar
Hirose, K, Amano, H, Baxter, MS, Chaykovskaya, E, Chumichev, VB, Hong, GH, Isogai, K, Kim, CK, Kim, SH, Miyao, T, Morimoto, T, Nikitin, A, Oda, K, Pettersson, HBL, Povinec, PP, Seto, Y, Tkalin, A, Togawa, O, Veletova, NK. 1999. Anthropogenic radionuclides in seawater in the East Sea/Japan Sea: Results of the first-stage Japanese-Korean-Russian expedition. Journal of Environmental Radioactivity 43:113.CrossRefGoogle Scholar
IAEA. 1986. Definition and recommendations for the convention on the prevention of marine pollution by dumping of wastes and other matter. IAEA Safety Series 78. Vienna: International Atomic Energy Agency.Google Scholar
IAEA. 1999. Inventory of radioactive waste disposals at sea. IAEA-TECDOC-1105. Vienna: International Atomic Energy Agency.Google Scholar
Ikeuchi, Y, Amano, H, Aoyama, M, Berezhnov, VI, Chaykovskaya, E, Chumichev, VB, Chung, CS, Gastaud, J, Hirose, K, Hong, GH, Kim, CK Kim, SH, Miyao, T, Morimoto, T, Nikitin, A, Oda, K, Pettersson, HBL, Povinec, PP, Tkalin, A, Togawa, O, Veletova, NK. 1999. Anthropogenic radionuclides in seawater of the Far Eastern Seas. The Science of the Total Environment 237/238:203212.Google Scholar
Jull, AJT, Burr, GS, Courtney, C, Povinec, PP, Togawa, O. 1999. Measurements of radiocarbon in the NW Pacific Ocean and its marginal seas. Proceedings of the International Symposium on Marine Pollution, Monaco, Oct. 5–9, 1998 IAEA-TECDOC-1094, Vienna, Austria: 249253.Google Scholar
Keeling, RF, Peng, TH. 1991. Transport of heat, CO2 and O2 by the Atlantic's thermohaline circulation. Philosophical Transactions of the Royal Society of London B 348:133142.Google Scholar
Key, RM. 1996. WOCE Pacific Ocean Radiocarbon Program. Radiocarbon 38(3):415423.Google Scholar
NEA. 1996. Coordinated research and environmental surveillance programme related to sea disposal of radioactive waste. CRESP Final Report 1991–1995. Paris: OECD.Google Scholar
Nyffeler, F, Cigna, AA, Dahlgaard, H, Livingston, HD. 1996. Radionuclides in the Atlantic Ocean: A Survey. In: Radionuclides in the oceans inputs and inventory. Guéguéniat, P, Germain, P, Métivier, H, coordinators. Institut de Protection et de Surete Nucleaire, Les Editions de Physique, FR, 29:128.Google Scholar
Östlund, HG, Dorsey, HG, Rooth, CG. 1974. GEOSECS North Atlantic radiocarbon and tritium results. Earth Planetary and Science Letters 23:6986.Google Scholar
Östlund, HG, Rooth, CGH. 1990. The North Atlantic tritium and radiocarbon transients 1972–1983. Journal of Geophysical Research 95 C 11:20,14720,165.Google Scholar
Pettersson, HBL, Amano, H, Berezhnov, VI, Chaykovskaya, E, Chumichev, VB, Chung, CS, Gastaud, J, Hirose, K, Hong, GH, Kim, CK, Kim, SH, Lee, SH, Morimoto, T, Nikitin, A, Oda, K, Povinec, PP, Suzuki, E, Tkalin, A, Togawa, O, Veletova, NK, Volkov, Y, Yoshida, K. 1999. Anthropogenic radionuclides in sediments in the NW Pacific Ocean and its marginal seas: results of the 1994–1995 Japanese-Korean-Russian expeditions. The Science of the Total Environment 237/238:213–24.CrossRefGoogle Scholar
Povinec, PP, Togawa, O. 1999. Marine radioactivity studies in World Oceans (MARS). Proceedings of the International Symposium on Marine Pollution, Monaco, Oct. 5-9, 1998 IAEA-TECDOC-1094, Vienna, Austria:262–68.Google Scholar
Schlitzer, R. 1986. 14C in the deep water of the East Atlantic. Radiocarbon 28 (2A):391396.Google Scholar
Seung, Y-H, Yoon, J-H. 1995. Some features of winter convection in the Japan Sea. Journal of Oceanography 51:6173.Google Scholar
Takahashi, T, Takahashi, TT, Sutherland, SC. 1995. An assessment of the role of the North Atlantic as a CO2 sink. Philosophical Transactions of the Royal Society of London B348:143152.Google Scholar
Tsunogai, S, Watanabe, YW, Harada, K, Watanabe, S, Saito, S, Nakajima, M. 1993. Dynamics of the Japan Sea deep waters studied with chemical and radiochemical tracers. In: Teramoto, T, editor. Deep ocean circulation, physical and chemical aspects. London: Elsevier. 105119.CrossRefGoogle Scholar