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Further Application of Bomb 14C as a Tracer in the Atmosphere and Ocean

Published online by Cambridge University Press:  18 July 2016

Reidar Nydal
Affiliation:
Radiological Dating Laboratory, The Norwegian Institute of Technology, N-7034 Trondheim NTH N-7034 Norway
Jorunn S. Gislefoss
Affiliation:
Radiological Dating Laboratory, The Norwegian Institute of Technology, N-7034 Trondheim NTH N-7034 Norway
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Abstract

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Bomb 14C from nuclear tests in the atmosphere has proved to be a particularly useful tool in the study of the carbon cycle. We provide here a ca. 30-yr time series of 14C concentrations in the atmosphere between 28°N and 71°N and in the ocean surface between 45°S and 45°N. More recently (since 1990), a north-south profile also has been obtained for 14C in the surface waters of the Atlantic Ocean. The measurements were performed using the conventional technique of beta counting or large samples (4 to 5 liter CO2) in CO2 proportional counters. These data show that the 14C concentration in the atmosphere is leveling off with a time constant of 0.055 yr-1, and is now approaching that of the ocean surface at lower latitudes.

Additional tracer studies have been concerned especially with the penetration of bomb 14C into the deep ocean. The Norwegian and Greenland seas are of interest as a sink for atmospheric CO2 and also a source of water for the deep Atlantic Ocean. During the last five years, several 14C depth profiles have been measured from the Fram Strait (79°N) to south of Iceland (62°N), using the AMS technique available at the University of Arizona AMS Facility. We considered it important to repeat and compare a few of the profiles with those produced by the GEOSECS expedition in 1972 and the TTO expedition in 1981. The profiles show that water descending to the deep Atlantic Ocean is originating mainly from intermediate and surface depths in the Nordic Seas. However, the ventilation rate of the Norwegian Sea deepwater is too slow to be an important component in the transfer of water over the Greenland-Scotland Ridge.

Type
14C Cycling and the Oceans
Copyright
Copyright © the Arizona Board of Regents on behalf of the University of Arizona 

References

REFERENCES

Bønisch, G. and Schlosser, P. 1995 Deep water formation and exchange rates in the Greenland/Norwegian Seas and the Eurasian Basin of the Arctic Ocean as derived from tracer balances. Progress in Oceanography 35: 2952.CrossRefGoogle Scholar
Bourke, R. H., Paquette, R. G., Blythe, R. F. and Stone, M. D. 1993 On the deep and bottom waters of the Greenland Sea from summer 1989 to 1990 data. Journal of Geophysical Research 98(C3): 46294638.CrossRefGoogle Scholar
Broecker, W. S. and Peng, T.-H. 1982 Tracers in the Sea. Palisades, New York, Eldigio Press: 690 p.Google Scholar
Broecker, W. S., Peng, T.-H., Östlund, G. and Stuiver, M. 1985 The distribution of bomb radiocarbon in the ocean. Journal of Geophysical Research 90(C4): 69536970.CrossRefGoogle Scholar
Donahue, D. J., Linick, T. W. and Jull, A. J. T. 1990 Isotope-ratio and background corrections for accelerator mass spectrometry radiocarbon measurements. Radiocarbon 32(2): 135142.CrossRefGoogle Scholar
Feely, H. W., Katzman, D. and Tucek, C. S. 1966 16th Progress Report Project Stardust, DASA.Google Scholar
Foldvik, A. and Gammelsrød, T. 1988 Notes on southern ocean hydrography, sea-ice and bottom water formation. Paleogeography, Paleoclimatology and Paleoecology 67: 317.CrossRefGoogle Scholar
Gislefoss, J. S. 1994 Carbon profiles in the Nordic Seas. PhD. dissertation, NTH-Trondheim: 170 p.Google Scholar
Gislefoss, J., Nydal, R., Donahue, D. J., Jull, A. J. T. and Toolin, L. J. 1994 Tracer studies of 14C in the Nordic Seas by AMS measurements. Nuclear Instruments and Methods in Physics Research B92: 431435.CrossRefGoogle Scholar
Gislefoss, J. S., Nydal, R., Skjelvan, I., Nes, A., Østerhus, S., Holmén, K., Jull, T. and Sonninen, E. 1995 Carbon profiles in the Nordic Seas. Data Report 2. Radiological Dating Laboratory, Trondheim, Tapir: 61 p.Google Scholar
Heinze, C., Schlosser, P., Koltermann, K. P. and Meincke, J. 1990 A tracer study of the deep water renewal in the European polar seas. Deep-Sea Research 37(9): 14251453.CrossRefGoogle Scholar
Levin, I., Graul, R. and Trivett, N. B. A. 1995 Long-term observations of atmospheric CO2 and carbon isotopes at continental sites in Germany. Tellus 47B (Series B): 2334.CrossRefGoogle Scholar
Linick, T. W., Jull, A J. T., Toolin, L. J. and Donahue, D. J. 1986 Operation of the NSF-Arizona Desolator Facility for Radioisotope Analysis and results from selected collaborative research projects. In Stuiver, M. and Kra, R. S., eds., Proceedings of the 12th International 14C Conference. Radiocarbon 28(2A): 522533.CrossRefGoogle Scholar
Mangerud, J. and Gulliksen, S. 1975 Apparent radiocarbon ages of recent marine shells from Norway, Spitsbergen and Arctic Canada. Quaternary Research 5: 263273.CrossRefGoogle Scholar
Meijer, H. A. J., van der Plicht, J., Gislefoss, J. S. and Nydal, R. 1994 Comparing long-term atmospheric 14C and 3H records near Groningen, The Netherlands with Fruholmen, Norway and Izaña, Canary Islands. Radiocarbon 37(1): 3950.CrossRefGoogle Scholar
Nakamura, T., Nakazawa, T., Nakai, N., Kitagawa, H., Honda, H., Itoh, T., Machida, T. and Matsumoto, E. 1992 Measurement of 14C concentrations of stratospheric CO2 by accelerator mass spectrometry. In Long, A. and Kra, R. S., eds., Proceedings of the 14th International 14C Conference. Radiocarbon 34(2): 745752.CrossRefGoogle Scholar
Nydal, R. 1968 Further investigation on the transfer of radiocarbon in nature. Journal of Geophysical Research 73(12): 36173635.CrossRefGoogle Scholar
Nydal, R. 1993 Application of bomb 14C as a tracer in the global carbon cycle. Trends in Geophysical Research 2: 355364.Google Scholar
Nydal, R., Gislefoss, J., Skjelvan, I., Blindheim, J., Foldvik, A., Vinje, T. and Østerhus, S. 1991 Measurements of carbon profiles in the Nordic seas. Norsk Polarinstitutt Rapportserie, Datareport 75: 143.Google Scholar
Nydal, R., Gislefoss, J., Skjelvan, I., Skogseth, F. H., Jull, A. J. T. and Donahue, D. J. 1992 14C profiles in the Norwegian and Greenland Seas by conventional AMS measurements. In Long, A. and Kra, R. S., eds., Proceedings of the 14th International 14C Conference. Radiocarbon 34(3): 717726.CrossRefGoogle Scholar
Nydal, R., Gulliksen, S., Løvseth, K. and Skogseth, F. H. 1984 Bomb 14C in the ocean surface, 1966–1981. Radiocarbon 26(1): 745.CrossRefGoogle Scholar
Nydal, R. and Løvseth, K. 1983 Tracing bomb 14C in the atmosphere 1962–1980. Journal of Geophysical Research 88(C6): 36213635.CrossRefGoogle Scholar
Östlund, H. G., Dorsey, H. G. and Brecher, R. (ms.) 1976 GEOSECS Atlantic, radiocarbon and tritium results. Data report from Rosenstiel School of Marine and Atmospheric Sciences. Florida, University of Miami: 93 p.Google Scholar
Östlund, H. G. and Rooth, C. G. H. 1990 The North Atlantic tritium and radiocarbon transients 1972–1983. Journal of Geophysical Research 95(C11): 20,14720,165.CrossRefGoogle Scholar
Pickard, G. L. and Emery, W. J. 1990 Descriptive Physical Oceanography. Oxford, Pergamon Press: 320 p.Google Scholar
Schlosser, P., Bønisch, G., Rhein, M. and Bayer, R. 1991 Reduction of deep-water formation in the Greenland Sea during the 1980s: Evidence from tracer data. Science 251: 10541056.CrossRefGoogle ScholarPubMed
SIPRI Yearbook 1975 World Armament and Disarmaments. Stockholm, Almqvist & Wiksell.Google Scholar
Slota, P. J. Jr., Jull, A. J. T., Linick, T. W. and Toolin, L. J. 1987 Preparation of small samples for 14C accelerator targets by catalytic reduction of CO. Radiocarbon 29(2): 303306.CrossRefGoogle Scholar
Smethie, W. M. Jr., Östlund, H. G., and Loosli, H. H. 1986 Ventilation of the deep Greenland and Norwegian seas: Evidence from krypton-85, tritium, carbon-14 and argon-39. Deep-Sea Research 33: 675703.CrossRefGoogle Scholar
Strass, V. H., Fairbach, E., Schauer, U. and Sellmann, L. 1993 Formation of Denmark Strait overflow water by missing the East Greenland Current. Journal of Geophysical Research 90(C4): 69076919.CrossRefGoogle Scholar
Stuiver, M. and Polach, H. A. 1977 Discussion: Reporting of 14C data. Radiocarbon 19(3): 355363.CrossRefGoogle Scholar
Swift, J. H., Aagaard, K. and Malmberg, S.-A. 1980 The contribution of the Denmark Strait overflow to the deep North Atlantic. Deep-Sea Research 27A: 2942.CrossRefGoogle Scholar
Swift, J. H. and Koltermann, K. P. 1988 The origin of Norwegian Sea deep water. Journal of Geophysical Research 93: 35633569.CrossRefGoogle Scholar
Tans, P. 1981 A compilation of bomb 14C data for use in global carbon model calculation. In Bolin, B., ed., Carbon Cycle Modeling. SCOPE: 390 p.Google Scholar
U.N. Report 1964 Radioactive contamination of the environment by nuclear tests, effect of atomic radiation. United Nations Scientific Committee Report 14 (A/5814): 120 p.Google Scholar