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Calculating Isotope Ratios and Nuclide Concentrations for In Situ Cosmogenic 14C Analyses

Published online by Cambridge University Press:  26 July 2016

Kristina Hippe*
Affiliation:
Laboratory of Ion Beam Physics, ETH Zürich, Otto-Stern-Weg 5, 8093 Zürich, Switzerland Institute of Geochemistry and Petrology, ETH Zürich, Clausiusstrasse 25, 8092 Zürich, Switzerland
Nathaniel A Lifton
Affiliation:
Department of Earth, Atmospheric, and Planetary Sciences and Department of Physics, Purdue University, 550 Stadium Mall Drive, West Lafayette, IN 47907, USA. Email: [email protected]
*
Corresponding author. Email: [email protected].

Abstract

In situ radiocarbon inorganic production and retention pathways are distinct from those of the more commonly used traditional organic/atmospheric 14C. In addition, a growing number of laboratories are extracting in situ cosmogenic 14C from quartz, using a variety of analytical techniques. As such, a flexible yet internally consistent set of procedures for data reduction that recognizes the unique nature of the in situ14C system is essential for reliable comparison of results among laboratories. This article thus presents a brief data reduction framework that can accommodate differences in both AMS and laboratory analytical techniques.

Type
Articles
Copyright
Copyright © 2014 by the Arizona Board of Regents on behalf of the University of Arizona 

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References

Bella, F, Alessio, M, Fratelli, P. 1968. A determination of the half-life of 14C. Il Nuovo Cimento Series B 58:232–46.Google Scholar
Coplen, T. 1996. New guidelines for reporting stable hydrogen, carbon, and oxygen isotope-ratio data. Geochimica et Cosmochimica Acta 60(17):3359–60.Google Scholar
Craig, H. 1957. Isotopic standards for carbon and oxygen and correction factors for mass-spectrometric analysis of carbon dioxide. Geochimica et Cosmochimica Acta 12(1–2):133–49.Google Scholar
Donahue, DJ, Linick, TW, Jull, AJT. 1990. Isotope-ratio and background corrections for accelerator mass spectrometry radiocarbon measurements. Radiocarbon 32(2):135–42.Google Scholar
Godwin, H. 1962. Half-life of radiocarbon. Nature 195(4845):984.Google Scholar
Goehring, BM, Schimmelpfennig, I, Schaefer, JM. 2014. Capabilities of the Lamont-Doherty Earth Observatory in situ 14C extraction laboratory updated. Quaternary Geochronology 19:194–7.Google Scholar
Gonfiantini, R, Stichler, W, Rozanski, K. 1995. Standards and materials distributed by the International Atomic Energy Agency for stable isotope measurements. In: Reference and Intercomparison Materials for Stable Isotopes of Light Elements. International Atomic Energy Agency TECDOC-825. Vienna: IAEA. p 1329.Google Scholar
Hippe, K, Kober, F, Baur, H, Ruff, M, Wacker, L, Wieler, R. 2009. The current performance of the in situ 14C extraction line at ETH. Quaternary Geochronology 4(6):493500.CrossRefGoogle Scholar
Hippe, K, Kober, F, Wacker, L, Fahrni, SM, Ivy-Ochs, S, Akçar, N, Schlüchter, C, Wieler, R. 2013. An update on in situ cosmogenic 14C analysis at ETH Zürich. Nuclear Instruments and Methods in Physics Research B 294:81–6.Google Scholar
Lal, D, Jull, AJT. 1994. Studies of cosmogenic in-situ 14CO and 14CO2 produced in terrestrial and extraterrestrial samples: experimental procedures and applications. Nuclear Instruments and Methods in Physics Research B 92(1–4):291–6.CrossRefGoogle Scholar
Lifton, NA. 1997. A new extraction technique and production rate estimate for in situ cosmogenic 14C in quartz [PhD dissertation]. Tucson: University of Arizona. 204 p.Google Scholar
Lifton, NA, Jull, AJT, Quade, J. 2001. A new extraction technique and production rate estimate for in situ cosmogenic 14C in quartz. Geochimica et Cosmochimica Acta 65(12):1953–69.Google Scholar
Mann, WB. 1983. An international reference material for radiocarbon dating. Radiocarbon 25(2):519–27.Google Scholar
Mann, WB, Marlow, WF, Hughes, EE. 1961. The half-life of carbon-14. International Journal of Applied Radiation and Isotopes 11:5767.CrossRefGoogle ScholarPubMed
Mook, WG, van der Plicht, J. 1999. Reporting 14C activities and concentrations. Radiocarbon 41(3):227–39.Google Scholar
Olsson, IU, Karlén, I, Turnbull, AH, Prosser, NJD. 1962. A determination of the half-life of C14 with a proportional counter. Arkiv för Fysik 22:237–55.Google Scholar
Reimer, PJ, Brown, TA, Reimer, RW. 2004. Discussion: reporting and calibration of post-bomb 14C data. Radiocarbon 46(3):1299–304.Google Scholar
Roberts, ML, Southon, JR. 2007. A preliminary determination of the absolute 14C/12C ratio of OX-I. Radiocarbon 49(2):441–5.Google Scholar
Stuiver, M. 1980. Workshop on 14C data reporting. Radiocarbon 22(3):964–6.Google Scholar
Stuiver, M. 1983. Business meeting: international agreements and the use of the new oxalic acid standard. Radiocarbon 25(2):793–5.Google Scholar
Stuiver, M, Polach, HA. 1977. Discussion: reporting of 14C data. Radiocarbon 19(2):355–63.CrossRefGoogle Scholar
Wacker, L, Christl, M, Synal, H-A. 2010. Bats: a new tool for AMS data reduction. Nuclear Instruments and Methods in Physics Research B 268(7–8):976–9.Google Scholar
Watt, DE, Ramsden, D, Wilson, HW. 1961. The half-life of Carbon-14. International Journal of Applied Radiation and Isotopes 11:6874.Google Scholar