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14C Variations Caused by Changes in the Global Carbon Cycle

Published online by Cambridge University Press:  18 July 2016

Ulrich Siegenthaler
Affiliation:
Physics Institute, University of Bern, Sidlerstrasse 5, 3012 Bern, Switzerland
Martin Heimann
Affiliation:
Physics Institute, University of Bern, Sidlerstrasse 5, 3012 Bern, Switzerland
Hans Oeschger
Affiliation:
Physics Institute, University of Bern, Sidlerstrasse 5, 3012 Bern, Switzerland
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Abstract

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A box-diffusion model for the carbon cycle is used to estimate the magnitude of 14C variations caused by changes of reservoir sizes and exchange fluxes in the global carbon system. The influence of changes in atmospheric CO2 concentration, biomass, CO2 exchange rate between atmosphere and ocean, and ocean mixing is considered. Steady-state 14C concentrations as well as the transients are calculated. For changing biomass, atmospheric CO2 levels and 13C/12C ratios are also calculated.

Carbon-cycle-induced 14C variations may have been significant in the transition period from Glacial to Postglacial when drastic changes in environmental conditions took place within short time periods, while they were probably less important during the climatically more stable Postglacial.

Changes of the oceanic circulation, as supposedly occurred, are considered the most important factor, besides variations of the production rate, affecting the global distribution of 14C. 14C variations due to changes of the atmospheric CO2 level or the air-sea-exchange probably did not exceed one to a few percent. Fluctuations of the forest biomass, which may have occurred between Glacial and Postglacial, hardly affected the 14C concentration over a long term.

Responses of the atmospheric 14C concentration are also calculated for variations of the 14C production rate by cosmic radiation. The following cases are considered: a step change, square-wave changes producing “wiggles”, and sinusoidal variations.

Type
Natural 14C Variations
Copyright
Copyright © The American Journal of Science 

References

Andersen, N R, and Malahoff, A, ed, 1977, The fate of fossil fuel CO2 in the oceans: New York, Plenum Press.Google Scholar
Barbetti, Mike and Flude, K, 1979, Geomagnetic variation during the late Pleistocene period and changes in the radiocarbon time scale: Nature, v 279, p 202205.Google Scholar
Berger, W H, 1977, Carbon dioxide excursions and the deep-sea record: aspects of the problem, in Anderson, N R and Malahoff, A, eds, The fate of fossil fuel CO2 in the oceans: New York, Plenum Press, p 505542.CrossRefGoogle Scholar
Berner, Werner, Oeschger, Hans, and Stauffer, Bernhard, 1980, Information on the CO2 cycle from ice core studies, in Stuiver, Minze and Kra, Renee, eds, Internatl radiocarbon conf, 10th, Proc: Radiocarbon, v 22, no. 2, p 227235.Google Scholar
Broecker, W S, 1971, Calcite accumulation rates and glacial to interglacial changes in oceanic mixing, in Turekian, K K, ed, The Late Cenozoic Glacial ages: New Haven, Yale Univ Press, p 239265.Google Scholar
Broecker, W S 1979, A revised estimate of the radiocarbon age of North Atlantic deep water: Jour Geophys Research, v 84, p 32183226.Google Scholar
Broecker, W S and Peng, T-H, 1974, Gas exchange rates between air and sea: Tellus, v 26, p 2135.CrossRefGoogle Scholar
CLIMAP, 1976, The surface of the Ice age earth: Science, v 191, p 11311137.Google Scholar
Ekdahl, C A and Keeling, C D, 1973, Atmospheric carbon dioxide and radiocarbon in the natural carbon cycle: I. Quantitative deductions from records at Mauna Loa observatory and at the South Pole, in Woodwell, G M and Pecan, E V, eds, Carbon and the biosphere: US Atomic Energy Commission, p 5185.Google Scholar
Elsasser, W, Ney, E P, and Winckler, J R, 1956, Cosmic-ray intensity and geomagnetism: Nature, v 178, p 1226.CrossRefGoogle Scholar
Gordon, A L and Taylor, H W, 1975, Heat and salt balance within the cold waters of the world ocean: Numerical models of ocean circulation: Natl Acad Sci.Google Scholar
Heimann, Martin, 1978, Ueber ein geophysikalisches Modell des globalen CO2—Kreislaufs: Diploma thesis, Physics Inst, Univ Bern.Google Scholar
Houtermans, J, 1966, On the quantitative relationships between geophysical parameters and the natural 14C inventory: Zeitschr Physik, v 193, p 112.Google Scholar
Jähne, B, Münnich, K O and Siegenthaler, Ulrich, 1979, Measurements of gas exchange and momentum transfer in a circular wind-water tunnel: Tellus, v 31, p 321329.Google Scholar
de Jong, A F M, Mook, W G, and Becker, Bernd, 1979, Confirmation of the Suess wiggles: 3200-3700 bc: Nature, v 280, p 4849.Google Scholar
Kanwisher, J, 1963, On the exchange of gases between the atmosphere and the sea: Deep Sea Research, v 10, p 195207.Google Scholar
Li, Y-H, Takahashi, T, and Broecker, W S, 1969, Degree of saturation of calcium carbonate in the oceans: Jour Geophys Research, v 74, p 55075525.CrossRefGoogle Scholar
Liss, P S and Slater, P G, 1974, Flux of gases across the air-sea interface: Nature, v 247, p 181184.Google Scholar
Oeschger, Hans, Siegenthaler, Ulrich, Gugelmann, A, and Schotterer, Ulrich, 1975, A box-diffusion model to study the carbon dioxide exchange in nature: Tellus, v 27, p 168192.Google Scholar
Olsson, I, ed, 1970, Radiocarbon variations and absolute chronology, Nobel symposium, 12th, Proc: Stockholm, Almqvist & Wiksell.Google Scholar
Reiter, E R, 1975, Stratospheric-tropospheric exchange processes: Rev Geophys Space Physics, v 13, p 459474.CrossRefGoogle Scholar
Ruddiman, W F and McIntyre, A, 1973, Time-transgressive deglacial retreat of polar waters from the North Atlantic: Quaternary Research, v 3, p 117130.Google Scholar
Schnitker, D, 1974, West Atlantic abyssal circulation during the past 120,000 years: Nature, v 248, p 385387.Google Scholar
Shackleton, N J, 1977, Carbon-13 in Uvigerina: Tropical rainforest history and the Equatorial Pacific carbonate dissolution cycles, in Andersen, N R and Malahoff, A, eds, The fate of fossil fuel CO2 in the oceans: New York, Plenum Press, p 401427.Google Scholar
Shackleton, N J, and Opdyke, N D, 1973, Oxygen isotope and palaeomagnetic stratigraphy of equatorial Pacific core V28-238: Oxygen isotope temperatures and ice volumes on a 105 year and 106 year scale: Quaternary Research, v 3, p 3355.CrossRefGoogle Scholar
Siegenthaler, Ulrich and Münnich, K O, in press, 13C fractionation during CO2 transfer from air to sea: SCOPE report on modeling of the global carbon cycle, in press.Google Scholar
Siegenthaler, Ulrich and Oeschger, Hans, 1978, Predicting future atmospheric carbon dioxide levels: Science, v 199, p 388395.Google Scholar
Streeter, S S and Shackleton, N J, 1979, Paleocirculation of the deep North-Atlantic: 150,000 year record of benthic foraminifera and oxygen-18: Science, v 203, p 168171.Google Scholar
Stuiver, Minze and Quay, P D, 1980, Changes in atmospheric carbon-14 attributed to a variable sun: Science, v 207, p 1119.Google Scholar
Suess, H E, 1968, Climatic changes, solar activity, and the cosmic-ray production rate of the natural radiocarbon: Meteorol Mon, v 8, p 146150.Google Scholar