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The Potential Role of Diffusion-Induced Grain-Boundary Migration in Extended Life Prediction

Published online by Cambridge University Press:  01 January 1992

C.A. Handwerker
Affiliation:
National Institute of Standards and Technology, Gaithersburg, MD 20899
J.E. Blendell
Affiliation:
National Institute of Standards and Technology, Gaithersburg, MD 20899
C.G. Interrante
Affiliation:
U.S. Nuclear Regulatory Commission, Washington, DC 20555
T.M. Ahn
Affiliation:
U.S. Nuclear Regulatory Commission, Washington, DC 20555
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Abstract

The selection of materials that are suitable for various high-level waste-packaging designs must reflect the need to meet requirements for long-term performance in repository environments that change with time. With this in mind, we examine how grain boundaries in materials are induced to migrate as a result of solute diffusion even at low temperatures, how the composition of the matrix material is changed significantly by this diffusion-induced grain boundary migration (DIGM), and how the changing microstructures and compositions during DIGM lead to major changes in materials performance, such as corrosion or embrittlement. Methods are discussed for prediction of the long-term behavior of materials affected by DIGM.

Type
Research Article
Copyright
Copyright © Materials Research Society 1993

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References

REFERENCES

1. Code, U.S., of Federal Regulations, “Disposal of High-Level Radioactive Waste in Geologic Repositories,” Section 113, Subpart E – Technical Criteria, part 60, Chapter I, Title 10, “Energy.”Google Scholar
2.“Technical Considerations for Evaluating Substantially Complete Containment of High-Level Waste Within the Waste Package,” Manaktala, H.K., Interrante, C.G., NUREG/CR-5638, December 1990.Google Scholar
3.“A Regulatory Perspective on Design and Performance Requirements for Engineered Systems in High-Level Waste,” Bernero, R.M., High Level Radioactive Waste Management, Proceedings of the Third International Conference, Vol. 1, American Nuclear Society, Inc., N.Y., N.Y., p.818.Google Scholar
4. Handwerker, C.A., in: Diffusion in Thin Films and Microelectronic Materials, edited by Gupta, D. and Ho, P., (Noyes Publications, Parkridge, New Jersey, 1988), pp. 245322.Google Scholar
5. King, A.H., Int. Mater. Rev. 32, 173 (1987).Google Scholar
6. Yoon, D.N., in: Annual Review of Materials Science, edited by Huggins, R.A., Giordmaine, J. A., and Wachtman, J.B. Jr., (Annual Reviews, Inc., Palo Alto Calif, 1989), pp. 4358.Google Scholar
7. Blendell, J.E., Handwerker, C.A., Kaysser, W.A. and Petzow, G., in: Surface and Interfaces in Ceramic and Ceramic-Metal Systems, Materials Science Research, edited by Pask, J. and Evans, A.G., (Plenum Press, 14, New York, 1981), pp.217226.Google Scholar
8. Gupta, D., Campbell, D.R. and Ho, P.S., in: Thin Films-Interdiffusion and Reaction, edited by Poate, J.M., Tu, K.N. and Mayer, J.W. (John Wiley, New York, 1978), pp.119160.Google Scholar
9. Baglin, J.E.E., and Poate, J.M., in: Thin Films-Interdiffusion and Reaction, edited by Poate, J.M., Tu, K.N. and Mayer, J.W. (John Wiley, New York, 1978), pp.305358.Google Scholar
10. Kirsch, R.G., Poate, J.M. and Eibschutz, M., Appl. Phys. Lett., 29. 772 (1976).Google Scholar
11. den Broeder, F.J.A., Acta Metal. 20, 319 (1972).Google Scholar
12. Tu, K.N., J.Appl.Phys. 48, 3400 (1977).Google Scholar
13. Hillert, M., and Purdy, G.R., Acta Metall. 26, 333 (1978).Google Scholar
14. Jeong, J.J., Yoon, D.N. and Kim, D.-Y, Ame, J.. Ceram. Soc. 73 2063 (1990).Google Scholar
15. Lee, H.-Y. and Kang, S.-J., Acta Metall. 38, 1307 (1990).Google Scholar
16. den Broeder, F.J.A. and Nakahara, S., Scripta Metall. 17, 399 (1983).Google Scholar
17. Nakahara, S., and den Broeder, F.J.A., Scripta Metall. 17, 607 (1983).Google Scholar
18. Metals Handbook, Vol. 3, Properties and Selection: Stainless Steels, Tool Materials, and Special-Purpose Metals, (A.S.M., Metals Park, Ohio, 1980).Google Scholar
19. Li, C. and Hillert, M., Acta Metal. 29, 1949 (1981).Google Scholar
20. Cahn, R.W., in: Recrystallization, Grain Growth and Texture, edited by Margolin, H., (A.S.M., Metals Park, Ohio, 1966), p.99.Google Scholar
21. Hillert, M., Scripta Metall. 17, 237 (1983).Google Scholar
22. Blendell, J.E., Handwerker, C.A., Shen, C., and Dang, N.-D., in: Ceramic Microstructures '86, edited by Pask, J. and Evans, A. G., (Plenum Press, New York, 1988) pp. 541548.Google Scholar
23. Rhee, W.-H., Song, Y.-D. and Yoon, D.N., Acta Metall. 35, 57 (1987).Google Scholar
24. Handwerker, C.A., Cahn, J.W., Yoon, D.N. and Blendell, J.E., in: Diffusion in Solids: Recent Developments, edited by dayananda, M. A. and Murch, G.E., (TMS/AIME Publication, Warrendale, PA 1985) pp. 275292.Google Scholar
25. Yoon, D.N., Cahn, J.W., Handwerker, C.A., Blendell, J.E. and Baik, Y.J., in: Interface Migration and Control of Microstructure, edited by Pande, C.S., Smith, D.A., King, A.H. and Walter, J., (ASM Press, Metals Park, Ohio, 1986) 113.Google Scholar
26. Rhee, W.-H., Handwerker, C.A., Yoon, D.N., in: Interfacial Structure, Properties, and Design, ed. Yoo, M.H., Clark, W.A.T. and Briant, C.L., (Mater. Res. Soc. Proc 122, Pittsburgh, PA 1988) pp. 205212.Google Scholar
27. Smigelskas, A.D. and Kirkendall, E.O., Trans. AIME, 171, 130 (1947).Google Scholar
28. Doo, V.Y. and Baluffi, R.W., Acta metall. 6. 428 (1958).Google Scholar
29. Matthews, J.W. and Crawford, J.L, Phil.Mag 11 977 (1965).Google Scholar
30. Rhee, W.-H., Handwerker, C.A. and Yoon, D.N., unpublished research.Google Scholar
31. Harrison, J.D. and Wagner, C. Acta Met. 7 722 (1959).Google Scholar
32. Kim, D.-Y., Handwerker, C.A. and Blendell, J.E., presented at the 1992 MRS Fall Meeting, Boston, MA, 1992 (unpublished).Google Scholar
33. Speich, G.R., Trans. AIME 242, 1359 (1968).Google Scholar
34. Sulonen, M.S., Acta metall. 12, 749 (1964).Google Scholar
35. Lee, K.-R., Baik, Y.J. and Yoon, D.N., Acta metall. 35, 2145 (1987).Google Scholar
36. Ostertag, C.P., SIMS - Untersuchungen zur Volumen -und Komgrenzenfremddiffusion von Indium in Kupfer, M.S.thesis Universitat Stuttgart, 1981.Google Scholar
37. Chen, F.S. and King, A.H., Met. Trans. A 21, 2363 (1990).Google Scholar
38. Bullen, D.B. and Gdowski, G.E., Survey of Degradation Modes of Candidate Materials for High-Level Radioactive-Waste Disposal Containers, Volume 1. Phase Stability, Lawrence Livermore National Laboratory Report, UCID-21362 Vol.1, 1988.Google Scholar
39. Hilert, M. and Lagneborg, R., J. Mat. Sci. 6, 208 (1971).Google Scholar
40. Tawancy, H.M., J. Mat. Sci., 16, 2883 (1981).Google Scholar
41. Schutz, R.W. and Hall, J.A., Optimization of Mechanical/Corrosion Properties of Ti Code-12 Plate and Sheet, Part I1: Thermomechanical Processing Effects (Stage II Final Report), Sandia National Laboratory Report, SAND–87-7171, 1988.Google Scholar
42. Liu, D., Miller, W.A. and Aust, K.T., Acta metall. mater. 37, 3367 (1989).Google Scholar
43. Purdy, G.R., in: Proc. An. Int. Conf. on Solid-Solid Phase Transformations (citing experimental results obtained from K. Tashiro), edited by Aaronson, H. I., Laughlin, D.E., Sekerka, R.F. and Wayman, C.M., pp.521546. (TMS/AlME, Philadelphia PA, 1982).Google Scholar