Hostname: page-component-586b7cd67f-dsjbd Total loading time: 0 Render date: 2024-11-23T15:49:03.995Z Has data issue: false hasContentIssue false
  • English
  • Français

On the mechanism of charge transfer between neutral and negatively charged nitrogen-vacancy color centers in diamond

Published online by Cambridge University Press:  07 March 2011

Vladimira Petrakova ,
Andrew Taylor ,
Irena Kratochvilova ,
Frantisek Fendrych ,
Petr Cigler ,
Miroslav Ledvina ,
Jan Kucka ,
Jan Stursa ,
Jan Ralis  and
Jiri Vacik
...Show all authors
Vladimira Petrakova
Affiliation:
Czech Technical University, Faculty of Biomedical Engineering, Kladno, Czech Republic;
Andrew Taylor
Affiliation:
Academy of Sciences of the Czech Republic, Institute of Physics, v.v.i, Prague, Czech Republic;
Irena Kratochvilova
Affiliation:
Academy of Sciences of the Czech Republic, Institute of Physics, v.v.i, Prague, Czech Republic;
Frantisek Fendrych
Affiliation:
Academy of Sciences of the Czech Republic, Institute of Physics, v.v.i, Prague, Czech Republic;
Petr Cigler
Affiliation:
Gilead Science and IOCB Research Center, Institute of Organic Chemistry and Biochemistry, v.v.i., Academy of Sciences of the Czech Republic, Prague, Czech Republic;
Miroslav Ledvina
Affiliation:
Gilead Science and IOCB Research Center, Institute of Organic Chemistry and Biochemistry, v.v.i., Academy of Sciences of the Czech Republic, Prague, Czech Republic;
Jan Kucka
Affiliation:
Institute of Nuclear Physics, Academy of Sciences of the Czech Republic, v.v.i, Rez near Prague, Czech Republic;
Jan Stursa
Affiliation:
Institute of Nuclear Physics, Academy of Sciences of the Czech Republic, v.v.i, Rez near Prague, Czech Republic;
Jan Ralis
Affiliation:
Institute of Nuclear Physics, Academy of Sciences of the Czech Republic, v.v.i, Rez near Prague, Czech Republic;
Jiri Vacik
Affiliation:
Institute of Nuclear Physics, Academy of Sciences of the Czech Republic, v.v.i, Rez near Prague, Czech Republic;
Milos Nesladek
Affiliation:
IMOMEC division, IMEC, Institute for Materials Research, University Hasselt, Diepenbeek, Belgium;
Get access

Abstract

The presented work aims for the development of optically-traceable intracellular nanodiamond sensors, where photoluminescence can be changed by biomolecular attachment/delivery event. High biocompatibility, small size and stable luminescence from its color centers, makes nanodiamond (ND) particles an attractive alternative to molecular dyes for drug-delivery and cell-imaging applications. In our work we study how the surface modification of ND can change ND luminescence spectra. This method can be used as a novel detection tool for remote monitoring of chemical processes in biological systems. We discuss photoluminescence (PL) spectra of oxidized and hydrogenated ND and a single crystal diamond, containing engineered NV centers. The hydrogenation of ND leads to quenching of NV- related luminescence and a PL shift due to changing of occupation from NV- to NV0 states. We model this effect using electrical potential changes at the diamond surface.

Keywords

diamondnanoscaleluminescence
Type
Research Article
Information
MRS Online Proceedings Library (OPL) , Volume 1282: Symposium A – Diamond Electronics and Bioelectronics—Fundamentals to Applications IV , 2011 , mrsf10-1282-a07-05
Copyright
Copyright © Materials Research Society 2011

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

References

REFERENCES

[1] Ho, D., ACS Nano 3, 12, 3825–3829 (2009)Google Scholar
[2] Fu, C. C., Lee, H. Y., Chen, K., Lim, T. S., Wu, H. Y., Lin, P. K., Wei, P. K., Tsao, P. H., Chang, H. C., Fann, W., Proc. Natl. Acad. Sci. USA 3, 104, 727–732 (2007)10.1073/pnas.0605409104Google Scholar
[3] Liu, K. K., Cheng, C. L., Chang, C. C., Chao, J. I., Nanotechnology 18 325120 (2007)Google Scholar
[4] Kreuger, A., J. Materials and Chemistry 18, 13, 1485–1492 (2008)10.1039/b716673gGoogle Scholar
[5] Davies, G., Hamer, M. F., Proc. R. Soc. Lond. A., 348, 285–298 (1976)10.1098/rspa.1976.0039Google Scholar
[6] Iakoubovskii, K., Adriaenssens, G. J., Nesladek, M., J. Phys.:Cond. Matter 12, 189–199 (2000)Google Scholar
[7] Ristein, J., Riedel, M., Ley, L., J. Electrochem. Soc., 151, 10, 315–321 (2004)10.1149/1.1785797Google Scholar
[8] Iakoubovskii, K., Adriaenssens, G. J., J. Phys.: Condens. Matter 13, 6015–18 (2001)Google Scholar
[9] Kratochvilova, , Taylor, A., Kovalenko, A., Fendrych, F., Rezacova, V., Petrak, V., Zalis, S., Sebera, J., Nesladek, M., Mater. Res. Soc. Symp. Proc., 1203, J03–05, (2010)Google Scholar
[10] Nesladek, M., Stals, L. M., Stesmans, A., Iakoubovskij, K., Adriaenssens, G. J., Appl. Phys. Lett., 72, 25, 3306–3308 (1998)Google Scholar
[11] Goss, J. P., Briddon, P. R., Jones, R., Sque, S., Rayson, M. J., Phys. Rev. B, 72, 035214 (2005)Google Scholar
[12] Ristein, J., Riedel, M., Stammler, M., Mantel, B. F., Ley, L., Diamond Relat. Mater., 11, 359–364 (2002)Google Scholar
[13] Santori, C., Barclay, P. E., Fu, K. C., Beausoleil, R. G., Phys. Rev. B, 79, 12, 5313–5321 (2009)Google Scholar
[14] Rezek, B., Sauerer, C., Nebel, C. E., Stutzmann, M., Ristein, J., Ley, L., Snidero, E., Bergonzo, P., Appl. Phys. Letters, 82, 14 (2003)Google Scholar