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Nonlinear Optical Defect Absorption in Hydrogenated Amorphous Silicon

Published online by Cambridge University Press:  15 February 2011

W. Rjeger
Affiliation:
Walter Schottky Institut, TU München, D-85748 Garching, Germany
M. Lanz
Affiliation:
Walter Schottky Institut, TU München, D-85748 Garching, Germany
C. F. O. Graeff
Affiliation:
Walter Schottky Institut, TU München, D-85748 Garching, Germany
C. E. Nebel
Affiliation:
Walter Schottky Institut, TU München, D-85748 Garching, Germany
M. Stutzmann
Affiliation:
Walter Schottky Institut, TU München, D-85748 Garching, Germany
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Abstract

By using a Nd: YAG-pumped optical parametric oscillator (OPO) as excitation light source (8 ns pulse width), the dynamic range of photothermal deflection spectroseopy (PDS) is increased by a factor up to 1000. This enables the study of nonlinear defect absorption in intrinsic, phosphorus and boron doped a-Si:H. To probe nonlinear absorption of defects, the intensity of the fundamental emission of the Nd:YAG (1064 nm) has been varied over three orders of magnitude. For intensities greater than 1024 photons/ (cm2s), a significant increase of a by a factor 1.4 in p-, 1.2 in i-, and 1.15 in n-a-Si:H is detected. From electron spin resonance (ESR) and transient photoconductivity experiments on intrinsic a-Si:H, a bleaching of the defect density by electron excitation into the conduction band is measured. A hole-like signature in the ESR spectra indicates that electrons from the valence band are excited into the defect band as well. The data are interpreted based on a model for IR-induced nonlinear optical effects.

Type
Research Article
Copyright
Copyright © Materials Research Society 1995

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References

REFERENCES

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