Hostname: page-component-586b7cd67f-2brh9 Total loading time: 0 Render date: 2024-11-23T15:12:01.939Z Has data issue: false hasContentIssue false
  • English
  • Français

New Perspectives for the Spent Nuclear Fuel Radionuclides Release Model in a Deep Geological Repository

Published online by Cambridge University Press:  19 October 2011

Christophe Poinssot ,
Cécile FERRY  and
Arnaud POULESQUEN
Christophe Poinssot
Affiliation:
[email protected], CEA - Nuclear Energy Division, Department of Physics and Chemistry, Service for the Studies of the Radionuclides Behaviour, CEA Saclay, BP11, GIF SUR YVETTE, F-91191, France, +33.1.6908.3260, +33.1.6908.5254
Cécile FERRY
Affiliation:
[email protected], CEA, Nuclear Energy Division, Department of Physics & Chemistry, Service for the Studies of the Radionuclides Behaviour, CEA SACLAY, BP.11, GIF SUR YVETTE, F-91650, France
Arnaud POULESQUEN
Affiliation:
[email protected], CEA, Nuclear Energy Division, Department of Physics & Chemistry, Service for the Studies of the Radionuclides Behaviour, CEA SACLAY, BP.11, GIF SUR YVETTE, F-91650, France
Get access

Abstract

Spent Nuclear Fuel (SNF) source terms are used to define the release rate of radionuclides (RN) in a direct disposal and to assess the performance of this waste form. They classically distinguish between two contributions: (i) the Instant Release Fraction (IRF) of RN which are directly leached when water contacts the fuel, (ii) the slow and long term release of RN which are embedded within the fuel matrix. Recent experimental results bring significant input in our understanding and assessment of both contributions. However, they have not yet been integrated in the definition of the SNF source term. This paper will present the impact on the RN source term of the latest results on the SNF long term evolution and the key remaining scientific issues.

Keywords

waste managementactinidegeologic
Type
Research Article
Information
MRS Online Proceedings Library (OPL) , Volume 985: Symposium NN – Scientific Basis for Nuclear Waste Management XXX , 2006 , 0985-NN02-06
Copyright
Copyright © Materials Research Society 2007

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

References

REFERENCES

1. Johnson, L.H., Garisto, N.C. and Stroes-Gascoyne, S. (1985), Proc. Waste Management 1985, 479.Google Scholar
2. Johnson, L., Ferry, C., Poinssot, C. (2005), J. Nucl. Mat., 346, 56–65.Google Scholar
3. Poinssot, C., Ferry, C., Grambow, B., Kelm, M., Spahiu, K., Martinez, A., Johnson, L., Cera, E., Pablo, J.de, Quinones, J., Wegen, D., Lemmens, K., McMenamin, T., Mat. Res. Soc. Symp. Proc, Scientific Basis for Nuclear Waste Management XXIX, 421–432.Google Scholar
4. Poinssot, C., Ferry, C., Lovera, P., Jégou, C., Gras, JM. (2005), J. Nucl. Mat., 346, 66–77.Google Scholar
5. Cachoir, C., Carbol, P., Cobos-Sabate, J., Glatz, J.P., Grambow, B., Lemmens, K., Martinez-Esparza, A., Mennecart, T., Ronchi, C., Rondinella, V., Serrano-Purroy, D., Spahiu, K., Wegen, D., Wiss, T. (2005), JRC-ITU-SCA-2005/01 technical report.Google Scholar
6. Poinssot, C., Lovera, P., Ferry, C., Gras, JM., (2003), Mat. Res. Soc. Symp. Proc Vol 757, Scientific basis for nuclear Waste Management XXVI, 35–42.Google Scholar
7. Ferry, C., Poinssot, C., Cappelaere, C., Desgranges, L., Jégou, C., Miserque, F., Piron, JP., Roudil, D., Gras, JM. (2006), Specific outcomes of the research on the spent fuel long term evolution in interim dry storage and deep geological disposal, Journal of Nuclear Materials, 352, 246–253.Google Scholar
8. Ferry, C., Piron, JP., Stout, R. (2006), Mat. Res. Soc. Symp. Proc Vol 985, Scientific basis for nuclear Waste Management XXX, this conference.Google Scholar
9. Ferry, C., Lovera, P., Poinssot, C., Garcia, P. (2005), Theoretical approaches of diffusion coefficient enhanced by alpha self irradiation in spent nuclear fuel, Journal of Nuclear Material, 346, 48–55.Google Scholar
10. Carbol, P., Cobos-Sabate, J., Glatz, J.P., Rondinella, V., Wegen, D., Wiss, T., Loida, A., Metz, V., Kienzler, B., Spahiu, K., Grambow, B., Quinones, J., Martinez-Esparza, A. (2005), SKB technical report TR-05-09.Google Scholar
11. Shoesmith, D., (2006), Mat. Res. Soc. Symp. Proc Vol 985, Scientific basis for nuclear Waste Management XXX, this conference. Google Scholar
12. Ferry, C., Poinssot, C. et al., (2005), Synthesis on the spent fuel long term evolution, CEA report R6084.Google Scholar
13. Robit, V., Poinssot, C., Vitorge, P., Grambow, B., Cui, D., Spahiu, K., Catalette, H. (2005), Mat. Res. Soc. Symp. Proc Vol 985, Scientific basis for nuclear Waste Management XXIX, 489–496.Google Scholar