Hostname: page-component-586b7cd67f-tf8b9 Total loading time: 0 Render date: 2024-11-25T15:19:32.707Z Has data issue: false hasContentIssue false
  • English
  • Français

Magnetoelectric properties of BST/LSMO particulate composites

Published online by Cambridge University Press:  08 July 2011

Juan Beltran-Huarac ,
R. Martinez  and
R. Palai
Juan Beltran-Huarac
Affiliation:
Department of Physics, University of Puerto Rico, San Juan, PR 00931, USA
R. Martinez
Affiliation:
Department of Physics, University of Puerto Rico, San Juan, PR 00931, USA
R. Palai
Affiliation:
Department of Physics, University of Puerto Rico, San Juan, PR 00931, USA
Get access

Abstract

Currently, ferroelectric and ferromagnetic particulate composites are receiving a great deal of interest due to their novel applications in microelectronic devices. Their excellent properties such as high relative dielectric constant, low dielectric loss, strong tunability, and ferromagnetism with colossal magnetoresistance can be controlled by manipulating both electric and magnetic fields. Ba0.7Sr0.3TiO3 /La0.67Sr0.33MnO3 (BST/LSMO) composite was prepared with 20:1 wt% by a high temperature solid-state reaction route. The X-ray diffraction (XRD) pattern confirmed the formation and the coexistence of both phases corresponding to BST and LSMO. High resolution field emission scanning electron microscope (FE-SEM) and energy dispersive X-ray spectroscopy (EDS) revealed a uniform distribution of the grain size throughout the surface of the sample and the presence of all the constituent elements with its esteemed reaction stoichiometry, respectively. In spite of the presence of both phases, only one transition peak was seen (50Hz-5MHz) around 295 K in dielectric measurement suggesting a nonlinear magnetoelectric coupling. The dielectric properties of BST/LSMO composite carried with different magnetic fields (0-1.7 T) show significant change in the BST dielectric behavior at low frequencies. The M-H curves at room temperature (RT) showed a drop in the saturation magnetization compared with pure LSMO is consistent with our composite structures.

Keywords

particulateferroelectricferromagnetic
Type
Research Article
Information
MRS Online Proceedings Library (OPL) , Volume 1368: Symposium WW – Multiferroic, Ferroelectric, and Functional Materials, Interfaces and Heterostructures , 2011 , mrss11-1368-ww08-01
Copyright
Copyright © Materials Research Society 2011

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

References

REFERENCES

[1] Spaldin, N. A. and Fiebig, M., Science (2005) 309: 391–392.Google Scholar
[2] Kimura, T., Goto, T., Shintani, H., Ishizaka, K., Arima, T. and Tokura, Y., Nature (2003) 426: 55–58.Google Scholar
[3] Eerenstein, W., Mathur, N. D. and Scott, J. F., Nature (2006) 442: 759–765.Google Scholar
[4] Fiebig, M., Lottermoser, T., Fröhlich, D., Goltsev, A. V. and Pisarev, R. V., Nature (2002) 419: 818–820.Google Scholar
[5] Wang, J., Neaton, J. B., Zheng, H., Nagarajan, V., Ogale, S. B., Liu, B., Viehland, D., Vaithyanathan, V., Schlom, D. G., Waghmare, U. V., Spaldin, N. A., Rabe, K. M., Wuttig, M., and Ramesh, R., Science (2003) 299, 1719.Google Scholar
[6] Palai, R., Katiyar, R.S., Schmid, H., Tissot, P., Clark, S. J., Robertson, J., Redfern, S.A.T., Catalan, G., and, Scott, J. F., Phy. Rev. B (2008) 77, 014110.Google Scholar
[7] Palai, R., Schmid, H., Scott, J.F., and Katiyar, R.S., Phy. Rev. B (2010) 81, 064110.Google Scholar
[8] Palai, R., Scott, J.F. and Katiyar, R.S., Phy. Rev. B (2010), 81, 024115.Google Scholar
[9] Yang, H., Wang, Y. Q., Wang, H., and Jia, Q. X., Appl. Phys. Lett.(2010) 96, 012909.Google Scholar
[10] Wodecka-Duś, B., Lisińska-Czekaj, A., Orkisz, T., Adamczyk, M., Osińska, K., Kozielski, L. and Czekaj, D., Materials science-Poland (2007) 25: 791–799.Google Scholar
[11] Martinez, R., Kumar, A., Palai, R. and Katiyar, R. S., MRS Symp. Proc. (2010) 1199.Google Scholar
[12] Mathews, M., "Structural and magnetic properties of epitaxial La0.67Sr0.33MnO3 films and nanostructures" (2007), the doctor’s degree at the University of Twente.Google Scholar
[13] http://www.ccp14.ac.uk/tutorial/crys/ Google Scholar
[14] http://www.ccp14.ac.uk/tutorial/lmgp/#chekcell Google Scholar
[15] Manfred Fiebig, J. Phys. D: Appl. Phys. (2005) 38: R123–R152.Google Scholar