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Decay-Series Disequilibrium Study of In Situ Long-Term Radionuclide Transport in Water-Rock Systems

Published online by Cambridge University Press:  10 February 2011

Shangde. Luo ,
Teh-Lung Ku ,
Robert Roback ,
Micheal Murrell  and
Travis L. McLing
Shangde. Luo
Affiliation:
Dept. of Earth Sciences, Univ. of Southern California, Los Angeles, CA 90089-0740, [email protected]
Teh-Lung Ku
Affiliation:
Dept. of Earth Sciences, Univ. of Southern California, Los Angeles, CA 90089-0740
Robert Roback
Affiliation:
SMSJ 514, Los Alamos National Laboratory, Los Alamos, NM 87545
Micheal Murrell
Affiliation:
SMSJ 514, Los Alamos National Laboratory, Los Alamos, NM 87545
Travis L. McLing
Affiliation:
Idaho National Engineering and Environmental Laboratory, Idaho Falls, ID 83415-2107
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Abstract

Uranium and thorium-series disequilibrium in nature permits the determination of many in-situ physico-chemical, geologic and hydrologic variables that control the long-term migration of radionuclides in geologic systems. It also provides site-specific, natural analog information valuable to the assessment of geologic disposal of nuclear wastes. In this study, a model that relates the decay-series radioisotope distributions among solution, sorbed and solid phases in water-rock systems to processes of water transport, sorption-desorption, dissolution-precipitation, radioactive ingrowth-decay, and α recoil is discussed and applied to a basaltic aquifer at the Idaho National Engineering and Environmental Laboratory (INEEL), Idaho.

Type
Research Article
Information
MRS Online Proceedings Library (OPL) , Volume 608: Symposium QQ – Scientific Basis for Nuclear Waste Management XXIII , 1999 , 217
Copyright
Copyright © Materials Research Society 2000

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References

REFERENCES

1 Krishnaswami, S., Graustein, W. C., Turekian, K. K., and Dowd, J. F., Water Resour. Res. 18, 1663–1675 (1982).Google Scholar
2 McKinley, I. G. and Alexander, W. R., J. Contaminant Hydrology 13, 249–259 (1993); Radiochimica Acta 74, 263-267 (1996).Google Scholar
3 Ku, T. L., Luo, S., Leslie, B. W., and Hammond, D. E., in Uranium Series Disequilibrium: Applications to Earth, Marine and Environmental Sciences, edited by Ivanovich, M. and Harmon, R. S. (Clarendon Press, Oxford, 1992), pp. 631–668; Radiochim. Acta 80, 219-223 (1998).Google Scholar
4 Murphy, W. M., in Sixth EC Natural Analogue Working Group Meeting, Proceedings of an international workshop held in Santa Fe, New Mexico, USA, edited by Maravic, H. von and Smellie, J. (European Commission, EUR16761, 1996), pp. 233–241.Google Scholar
5 Luo, S., Ku, T. L., Roback, R., Murrell, M., and McLing, T. L., Geochim. Cosmochim. Acta (in press).Google Scholar
6 Knobel, L. L., Cecil, L., S., T. and , Wood, U. S. Geological Survey Open-File Report 95-748, Idaho Falls, Idaho, 1995.Google Scholar
7 Zukin, J. G., Hammond, D. E., Ku, T. L., and Elder, W. A., Geochim. Cosmochim. Acta 51, 1719–1931.Google Scholar
8 Wood, W. W. and Low, W. H., Geol. Soc. Amer. Bull. 97, 1456–1466 (1986).Google Scholar
9 Ackerman, D. J., U. S. Geological Survey Water Resources Investigations Report 94-4257, Idaho Falls, Idaho, 1995.Google Scholar