Hostname: page-component-cd9895bd7-mkpzs Total loading time: 0 Render date: 2024-12-27T02:02:20.335Z Has data issue: false hasContentIssue false
  • English
  • Français

Coupling of single DBT molecules to a graphene monolayer: proof of principle for a graphene nanoruler

Published online by Cambridge University Press:  23 February 2015

G. Mazzamuto ,
A. Tabani ,
S. Pazzagli ,
S. Rizvi ,
A. Reserbat-Plantey ,
K. Schädler ,
G. Navickaite ,
L. Gaudreau ,
F.S. Cataliotti  and
F. Koppens
...Show all authors
G. Mazzamuto
Affiliation:
LENS and Università di Firenze, Via Nello Carrara 1, I-50019 Sesto Fiorentino, Italy
A. Tabani
Affiliation:
LENS and Università di Firenze, Via Nello Carrara 1, I-50019 Sesto Fiorentino, Italy
S. Pazzagli
Affiliation:
LENS and Università di Firenze, Via Nello Carrara 1, I-50019 Sesto Fiorentino, Italy
S. Rizvi
Affiliation:
LENS and Università di Firenze, Via Nello Carrara 1, I-50019 Sesto Fiorentino, Italy
A. Reserbat-Plantey
Affiliation:
ICFO-Institut de Ciencies Fotoniques, Mediterranean Technology Park, E-08860 Castelldefels, Barcelona, Spain
K. Schädler
Affiliation:
ICFO-Institut de Ciencies Fotoniques, Mediterranean Technology Park, E-08860 Castelldefels, Barcelona, Spain
G. Navickaite
Affiliation:
ICFO-Institut de Ciencies Fotoniques, Mediterranean Technology Park, E-08860 Castelldefels, Barcelona, Spain
L. Gaudreau
Affiliation:
ICFO-Institut de Ciencies Fotoniques, Mediterranean Technology Park, E-08860 Castelldefels, Barcelona, Spain
F.S. Cataliotti
Affiliation:
LENS and Università di Firenze, Via Nello Carrara 1, I-50019 Sesto Fiorentino, Italy Dipartimento di Fisica ed Astronomia, Via Sansone 1, I-50019 Sesto Fiorentino, Italy QSTAR, Largo Enrico Fermi 2, I-50125 Firenze, Italy
F. Koppens
Affiliation:
ICFO-Institut de Ciencies Fotoniques, Mediterranean Technology Park, E-08860 Castelldefels, Barcelona, Spain
C. Toninelli*
Affiliation:
LENS and Università di Firenze, Via Nello Carrara 1, I-50019 Sesto Fiorentino, Italy QSTAR, Largo Enrico Fermi 2, I-50125 Firenze, Italy INO, Istituto Nazionale di Ottica, Largo Fermi 6, I-50125 Firenze, Italy
*
*E-mail: [email protected]
Get access

Abstract

We report on our recent progress in the study of single Dibenzoterrylene (DBT) molecules as single photon sources and nanoscale probes. We consider DBT molecules embedded in thin anthracene films, a system that allows stable single photon emission both at room and at cryogenic temperatures. We investigate the most important optical properties of the DBT:anthracene system as a whole. We then perform a full statistical study of the coupling between single DBT molecules by measuring the lifetimes of DBT both in the coupled and in the uncoupled case. The experimental results are framed into a simple universal scaling model, where the magnitude of coupling depends solely on universal parameters and on the distance d between the single emitter and the graphene monolayer. We apply this model to infer d and provide a proof of principle for a position ruler at the nanoscale [1].

Keywords

sensorthin filmphotoemission
Type
Articles
Information
MRS Online Proceedings Library (OPL) , Volume 1728: Symposium L – Optical Metamaterials and Novel Optical Phenomena Based on Nanofabricated Structures , 2015 , mrsf14-1728-l06-02
Copyright
Copyright © Materials Research Society 2015 

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

References

REFERENCES

Mazzamuto, G., Tabani, A., Pazzagli, S., Rizvi, S., Reserbat-Plantey, A., Schädler, K., Navickaite, G., Gaudreau, L., Cataliotti, F.S., Koppens, F. and Toninelli, C.. New Journal of Physics. 16 113007 (2014).10.1088/1367-2630/16/11/113007CrossRefGoogle Scholar
Nicolet, A. A. L., Bordat, P., Hofmann, C., Kol’chenko, M. A., Kozankiewicz, B., Brown, R. and Orrit, M.. Chem. Phys. Chem. 8 1929–36 (2007)10.1002/cphc.200700340CrossRefGoogle Scholar
Toninelli, C., Early, K., Bremi, J., Renn, A., Götzinger, S. and Sandoghdar, V.. Opt. Express 18 6577–682 (2010)10.1364/OE.18.006577CrossRefGoogle Scholar
Toninelli, C., Delley, Y., Stöferle, T., Renn, A., Götzinger, S. and Sandoghdar, V.. Appl. Phys. Lett. 97 021107 (2010)10.1063/1.3456559CrossRefGoogle Scholar
Nicolet, A. A. L., Bordat, P., Hofmann, C., Kol’chenko, M. A., Kozankiewicz, B., Brown, R. and Orrit, M.. Chem. Phys. Chem. 8 1929–36 (2007)10.1002/cphc.200700340CrossRefGoogle Scholar
Trebbia, J-B., Ruf, H., Tamarat, P. and Lounis, B.. Opt. Express. 17 23986–91 (2009)10.1364/OE.17.023986CrossRefGoogle Scholar
Moerner, W. E. and Orrit, M.. Science 283 1670–6 (1999)10.1126/science.283.5408.1670CrossRefGoogle Scholar
Michaelis, J., Hettich, C., Zayats, A., Eiermann, B., Mlynek, J. and Sandoghdar, V.. Opt. Lett. 24 581–3 (1999)10.1364/OL.24.000581CrossRefGoogle Scholar
Veerman, J. A., Garcia-Parajo, M. F., Kuipers, L. and van Hulst, N. F.. J. Microsc. 194 477–82 (1999)10.1046/j.1365-2818.1999.00520.xCrossRefGoogle Scholar
Homola, J., Yee, S. S. and Gauglitz, G.. Sensors Actuators B 54 3–15 (1999)10.1016/S0925-4005(98)00321-9CrossRefGoogle Scholar
O'Brien, J. L., Furusawa, A. and Vuckovic, J.. Nat. Photonics 3 687–95 (2009)10.1038/nphoton.2009.229CrossRefGoogle Scholar
Castro Neto, A. H., Guinea, F., Peres, N. M. R., Novoselov, K. S. and Geim, A. K.. Rev. Mod. Phys. 81 109–62 (2009)10.1103/RevModPhys.81.109CrossRefGoogle Scholar
Koppens, F. H. L., Chang, D. E. and García de Abajo, F. J.. Nano Lett. 11 3370–77 (2011)10.1021/nl201771hCrossRefGoogle Scholar
Chen, Z., Berciaud, S., Nuckolls, C., Heinz, T. F. and Brus, L. E.. ACS Nano 4 2964–68 (2010)10.1021/nn1005107CrossRefGoogle Scholar
Gaudreau, L., Tielrooij, K. J., Prawiroatmodjo, G. E. D. K., Osmond, J., García de Abajo, F. J. and Koppens, F. H. L.. Nano Lett. 13 2030–35 (2013)10.1021/nl400176bCrossRefGoogle Scholar
Lieb, M. A., Zavislan, J. M., and Novotny, L.. J. Opt. Soc. Am. B 21, 1210–1215 (2004).10.1364/JOSAB.21.001210CrossRefGoogle Scholar
Kreiter, M., Prummer, M., Hecht, B. and Wild, U. P.. J. Chem. Phys. 117 9430–33 (2002)10.1063/1.1515732CrossRefGoogle Scholar
Rogobete, L. and Henkel, C.. Phys. Rev. A 70 063815 (2004)10.1103/PhysRevA.70.063815CrossRefGoogle Scholar
Blanco, L. A. and García de Abajo, F. J.. Phys. Rev. B 69 205414 (2004)10.1103/PhysRevB.69.205414CrossRefGoogle Scholar
Glauber, R. J. and Lewenstein, M.. Phys. Rev. A 43 467– 91 (1991)10.1103/PhysRevA.43.467CrossRefGoogle Scholar
Treossi, E., Melucci, M., Liscio, A., Gazzano, M., Samorì, P. and Palermo, V.. J. Am. Chem. Soc. 131 15576–77 (2009)10.1021/ja9055382CrossRefGoogle Scholar
Tisler, J., Oeckinghaus, T., Stöhr, R. J., Kolesov, R., Reuter, R., Friedemann, R. and Wrachtrup, J.. Nano Lett. 13 3152–56 (2013)10.1021/nl401129mCrossRefGoogle Scholar
Liu, X., Wang, G., Song, X., Feng, F., Zhu, W., Lou, L., Wang, J., Wang, H. and Bao, P.. Appl. Phys. Lett. 101 233112 (2012)10.1063/1.4769367CrossRefGoogle Scholar
Gomez-Santos, G. and Stauber, T.. Phys. Rev. B 84 165438 (2011)10.1103/PhysRevB.84.165438CrossRefGoogle Scholar