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Uraninites of the Oklo Reactors: O Isotopes and Mineralogical Data

Published online by Cambridge University Press:  10 February 2011

L. Pourcelot
Affiliation:
Centre de Géochimie de la Surface-CNRS, 1, rue Blessig F67084 STRASBOURG, France
F. Gauthier-Lafaye
Affiliation:
Centre de Géochimie de la Surface-CNRS, 1, rue Blessig F67084 STRASBOURG, France
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Extract

Natural fission reactors located in the uranium ore deposits of Oklo-Okélobondo and Bangombé (Gabon) are a unique case of natural nuclear waste disposal. The Reactor Zones (RZ) (up to fifteen) cores are made of 60% uranium (UO2) embedded in a clay matrix [1]. The uraninites are depleted in 235U and contain fission products. Therefore, they are considered to be good analogues for spent nuclear fuel matrix [2]. The aim of this work is to study the conditions of preservation over a long periode of time of the uraninites which have been sumitted to interraction with fluid having different oxidizing potential. For this purposes mineralogical (X-ray powder diffraction), chemical (electron microprobe) and oxygen isotopic analyses were performed on uraninites from various RZs.

Type
Research Article
Copyright
Copyright © Materials Research Society 1998

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References

REFERENCES

1 Gauthier-Lafaye, F., Holliger, P. and Blanc, P. L., Geoch. et Cosmoch. Acta 60, p. 4831 (1996).Google Scholar
2 Janeczek, J., Ewing, R. C., Oversby, V. M. and Werme, L. O., J. Nucl. Mat. 238, p. 121 (1996).Google Scholar
3 Zheng, Y. F., Nucl. Sci. Tech. 6, p. 193 (1995).Google Scholar
4 Louvat, D., Toulhoat, P.., Smellie, J., Oklo Working Group, Proceeding of the fourth joint EC-CEA progress and final meeting, Saclay, France, p. 113126 (1995).Google Scholar
5 Bruno, J., Cera, E., Duro, L.., Eriksen, T.E., Werme, L.O., J. Nucl. Mater. 238, p. 110 (1996).Google Scholar
6 Kyser, T.G., Kotzer, T.K., Americ. Min. 78, p. 1262 (1993).Google Scholar
7 Pourcelot, L., PhD thesis dissertation, Université Strasbourg ULP France, 200 p. (1997).Google Scholar