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Radionuclide Migration into Natural Fracture Surfaces of Granitic Rock

Published online by Cambridge University Press:  21 February 2011

B. Torstenfelt
Affiliation:
Department of Nuclear Chemistry, Chalmers University of Technology, S–412 96 Göteborg, Sweden.
T. Eliasson
Affiliation:
Department of Nuclear Chemistry, Chalmers University of Technology, S–412 96 Göteborg, Sweden.
B. Allard
Affiliation:
Department of Nuclear Chemistry, Chalmers University of Technology, S–412 96 Göteborg, Sweden.
K. Andersson
Affiliation:
Department of Nuclear Chemistry, Chalmers University of Technology, S–412 96 Göteborg, Sweden.
S. Hoglund
Affiliation:
Department of Nuclear Chemistry, Chalmers University of Technology, S–412 96 Göteborg, Sweden.
T. Ittner
Affiliation:
Department of Nuclear Chemistry, Chalmers University of Technology, S–412 96 Göteborg, Sweden.
U. Olofsson
Affiliation:
Department of Nuclear Chemistry, Chalmers University of Technology, S–412 96 Göteborg, Sweden.
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Abstract

The uptake of cesium on natural fracture surfaces taken from granitic bedrock has been studied as well as the depth penetration into the underlying rock. The fracture minerals usually exhibit good sorptive properties with respect to cesium (with the exception of calcite). The surface coatings do not act as physical diffusion barriers and do not prevent a migration into the underlying rock. A considerable depth penetration into the rock (several mm over a period of three months) was observed. The dominating pathways into the rock matrix were the high-capacity minerals in grains or in microfissures. The calculated diffusivity in the rock matrix was of the order of 1013 m2/s.

Type
Research Article
Copyright
Copyright © Materials Research Society 1983

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References

REFERENCES

1. “Handling of Spent Nuclear Fuel and Final Storage of Vitrified High Level Reprocessing Waste” and “Handling and Final Storage of Unreprocessed Spent Nuclear Fuel”, Kärnbränslesäkerhet (KBS), (Stockholm 1977 and 1978).Google Scholar
2. Larson, S.A.. Tullborg, E.L. and Lindblom, S., “Sprickmineralogiska undersökningar”, (Studies of fracture mineralogy), PRAV 4.20, Programradet för radioaktivt avfall, (Stockholm 1981) (in Swedish).Google Scholar
3. Hultberg, B., Larson, S.A. and Tullborg, E.L., “Grundvatten i kristallin berggrund”, (Groundwater in crystalline bedrock), SGU Dnr 41.41.–81–H206- U, Swedish Geologic Survey, (Uppsala 1981).Google Scholar
4. Landstrbm, O., Klockars, C.E., Persson, O., Andersson, K., Torstenfelt, B., Allard, B., Larson, S.A. and Tullborg, E.L., “A Comparison of In-Situ Radionuclide Migration Studies in the Studsvik Area and Laboratory Measurements”, in Lutze, W. (Ed.), Scientific Basis for Nuclear Waste Management, Vol. 5, (Elsevier, New York), in press.Google Scholar
5. Andersson, K., Torstenfelt, B. and Allard, B., “Diffusion of Cesium in Concrete”, in Moore, J.G. (Ed.), Scientific Basis for Nuclear Waste Management. Vol. 3, (Plenum Publ. Corp., New York 1981) pp. 235242.Google Scholar
6. Torstenfelt, B., Allard, B. and Andersson, K., “Mobilities of Radionuclides in Fresh and Fractured Crystalline Rocks”, KBS-Technical Report, in prep.Google Scholar
7. Crank, J., The Mathematics of Diffusion, Second edition, (Oxford University Press, Oxford 1975).Google Scholar
8. Torstenfelt, B., Andersson, K. and Allard, B., Chem. Geol. 36, 123 (1982).Google Scholar
9. Allard, B., Larsson, S.A., Albinsson, Y., Tullborg, E.L., Karlsson, M., Andersson, K. and Torstenfelt, B., “Minerals and Precipitates in Fractures and Their Effects on the Retention of Radionuclides in Crystalline Rocks”, Proc. OECD/NEA Workshop on Near-field Phenomena in Geologic Repositories for Radioactive Waste, (OECD, Paris 1982) pp. 93100.Google Scholar
10. Andersson, K., Torstenfelt, B. and Allard, B., “Sorption Behaviour of Longlived Radionuclides in Igneous Rock”, in Migration in the Terrestrial Environment of Long-lived Radionuclides from the Nuclear Fuel Cycle, (IAEA, Vienna 1982) pp. 111131.Google Scholar
11. Neretnieks, I., J. Geophys. Res. 85, 4379 (1980).Google Scholar
12. Torstenfelt, B., Kipatsi, H., Andersson, K., Allard, B. and Olofsson, U., “Transport of Actinides Through a Bentonite Backfill”, in Lutze, W. (Ed.), Scientific Basis for Nuclear Waste Management, Vol. 5, (Elsevier, New York), in press.Google Scholar