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Natural Radionuclides in Hanford Site Ground Waters

Published online by Cambridge University Press:  28 February 2011

M. R. Smith
Affiliation:
Pacific Northwest Laboratory(a), P. O. Box 999, Richland, WA 99352
J. C. Laul
Affiliation:
Pacific Northwest Laboratory(a), P. O. Box 999, Richland, WA 99352
V. G. Johnson
Affiliation:
Westinghouse Hanford Corporation, P. O. Box 800, Richland, WA 99352
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Abstract

Uranium, Th, Ra, Rn, Pb and Po radionuclide concentrations in ground waters from the Hanford Site indicate that U, Th, and Ra are highly jorbed. Relative to Rn, these radionuclides are low by factors of 10−3 to 10−6. Uranium sorption is likely due to its reduction from the +6 state, where it is introduced via surface waters, to the +4 state found in the confined aquifers. The distribution of radionuclides is very similar in all of the confined aquifers and significantly different from the distribution observed in the unconfined and surface waters. Barium correlates well with Ra over three orders of magnitude indicating that stable element analogs may be useful for inferring the behavior of radioactive waste radionuclides in this candidate geologic repository.

Type
Research Article
Copyright
Copyright © Materials Research Society 1988

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References

1. Hubbard, N., Laul, J.C., and Perkins, R.W., “The Use of Natural Radionuclides to Predict the Behavior of Radwaste Radionuclides in Far-Field Aquifers,” Scientific Basis for Radioactive Waste Management VII, Mat. Res. Soc. Smp. Proc., Vol. 26, 891897, (1984).Google Scholar
2. Laul, J.C., Smith, M.R., Johnson, V.G., and Smith, R.M., “Disequilibrium of Natural Radionuclides in Hanford Site Ground Waters,” High Level Nuclear Waste Disposal Technology and Engineering, Ed. Burkholder, , 401–410, (1985).Google Scholar
3. Laul, J.C., Smith, M.R., Thomas, C.W., Jackson, P.O. and Hubbard, N., Analysis of Natural Radionuclides from Uranium and Thorium Series in Briny Groundwaters,” J. of Radioana. and Nucl. Chem., Articles, Vol. 110, No. 1, 101112, (1987).Google Scholar
4. Yang, I.C., “Improved Methods for the Determination of Dissolved Radium-226,” Proceedings of the Fifth International Conference on Nuclear Methods in Environmental and Energy Research, April 1–6, Mayaquez, Puerto Rico, p. 191, (1985).Google Scholar
5. Apps, J., Doe, T., Doty, B., Doty, S., Galbraith, R., Kearns, A., Kohrt, B., Lons, J., Monroe, A., Narasimhan, T.N., Nelson, P., Wilson, C.R., and Witherspoon, P.A., “Geohydrologic Studies for Nuclear Waste Isolation at the Hanford Reservation, LBL-8764, Vol. 2, Lawrence Berkeley Laboratory, Berkeley, California. (1979)Google Scholar
6. Grindler, J.E., “The Radiochemistry of Uranium,” Nuclear Science Series, NAS-NS, 3050, (1962).Google Scholar
7. Hyde, E.K., “The Radiochemistry of Thorium,” Nuclear Science Series, NAS-NS, 3004, (1960).Google Scholar
8. Early, T.O., Spice, G.D. and Mitchell, M.D., “A Hydrochemical Data Base for the Hanford Site, Washington,” SD-BWI-DP-061 Rev. 1, Rockwell Hanford Operations, Richland, Washington. (1986)Google Scholar