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Main results of the French program on Partitioning and Transmutation of Minor Actinides

Published online by Cambridge University Press:  27 March 2012

Ch. Poinssot
Affiliation:
CEA, Nuclear Energy Division, RadioChemistry & Processes Department, BP17171, F-30207 Bagnols sur Cèze, France, contact author: [email protected]
B Boullis
Affiliation:
CEA, Nuclear Energy Division, Nuclear Innovation and Support Program Division, CEA Saclay, F-91919 Gif sur Yvette cedex, France.
C. Rostaing
Affiliation:
CEA, Nuclear Energy Division, RadioChemistry & Processes Department, BP17171, F-30207 Bagnols sur Cèze, France, contact author: [email protected]
D. Warin
Affiliation:
CEA, Nuclear Energy Division, Nuclear Innovation and Support Program Division, CEA Saclay, F-91919 Gif sur Yvette cedex, France.
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Abstract

In the framework of the successive 1991 and 2006 Waste Management Act, French government supported a very significant R&D program on partitioning and transmutation of minor actinides (MA). This program aims to study potential solutions for still minimizing the quantity and the hazardousness of final waste, by MA recycling. Indeed, MA recycling can reduce the heat load and the half-life of most of the waste to be buried to a couple of hundred years, overcoming the concerns of the public related to the long-life of the waste.

Within this framework, this paper aims to present the most recent progress obtained in CEA on the development of innovative actinide partitioning hydrometallurgical processes in support of their recycling, either in an homogeneous mode (MA are recycled at low concentration in all the standard reactor fuel) or in an heterogeneous mode (MA are recycled at higher concentration in specific targets, at the periphery of the reactor core). Recovery performances obtained on recent tests in high active conditions of the so-called GANEX and DIAMEX-SANEX process will be presented and discussed in light of the potential P&T scenarios. Finally, recent developments regarding the recycling of the sole Am will be presented as well as the results obtained on highly active solutions for this so-called EXAM process.

This set of results gives to the French government a portfolio of potential recycling processes which could be separately and progressively implemented if decided.

Type
Articles
Copyright
Copyright © Materials Research Society 2012

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References

REFERENCES

1. Warin, D. and Courtois, C., “Overview of French P and T program and results for waste management”, 8th OECD/NEA International Exchange Meeting on P and T, Las Vegas, USA, (2004)Google Scholar
2. Courtois, C. et al. ., “High level radioactive waste / Research and results, Law of 30 december, 1991/Direction 1CEA Report DEN/DDIN/2005-568, (2005).Google Scholar
3. Rostaing, C. et al. ., Minor actinides partitioning: main results during the fifteen years research and prospects, ENC 2007, Brussels, Belgium (2007).Google Scholar
4. The French R&D Programme on the Partitioning and Transmutation of Long-Lived Radionuclides, An International Peer Review, OECD/NEA N°6210, ISBN 92-64-02296-1, (2006).Google Scholar
5. Heres, X. et al. . “Results of recent counter-current tests on AN (III)/Ln(III) separation using TODGA extractant”, Proceedings Global 2009, Paris, France (2009).Google Scholar
6. Miguirditchian, M. et al. . “HA demonstration in the Atalante facility of the Ganex 1st cycle for the selective extraction of Uranium from HLW”, Proceedings Global 2009, Paris, France (2009).Google Scholar
7. Miguirditchian, M. et al. . “HA demonstration in the Atalante facility of the Ganex 2nd cycle for the grouped TRU extraction”, Proceedings Global 2009, Paris, France (2009).Google Scholar
8. Warin, D.Future nuclear fuel cycles: prospect and challenges for actinide recycling”, Proceedings of the Actinide 2009 Conference, San Francisco, USA (2009).Google Scholar
9. Rostaing, C.Advanced processes for minor actinides recycling: studies towards potential industrialization”, Proceedings Global 2009, Paris, France (2009).Google Scholar