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Linear and Circular Dichroism in Angle Resolved Fe 3p Photoemission

Published online by Cambridge University Press:  15 February 2011

E. Tamura ,
G. D. Waddill ,
J. G. Tobin  and
P. A. Sterne
E. Tamura
Affiliation:
Lawrence Livermore National Laboratory, University of California, Livermore, CA 94550
G. D. Waddill
Affiliation:
Lawrence Livermore National Laboratory, University of California, Livermore, CA 94550
J. G. Tobin
Affiliation:
Lawrence Livermore National Laboratory, University of California, Livermore, CA 94550
P. A. Sterne
Affiliation:
Lawrence Livermore National Laboratory, University of California, Livermore, CA 94550 Department of Physics, University of California, Davis, CA 95616
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Abstract

Using a recently developed spin-polarized, fully relativistic, multiple scattering approach based on the layer KKR Green function method, we have reproduced the Fe 3p angle-resolved soft x-ray photoemission spectra and analyzed the associated large magnetic dichroism effects for excitation with both linearly and circularly polarized light. Comparison between theory and experiment yields a spin-orbit splitting of 1.0 – 1.2 eV and an exchange splitting of 0.9 – 1.0 eV for Fe 3p. These values are 50 – 100 % larger than those hitherto obtained experimentally.

Type
Research Article
Information
MRS Online Proceedings Library (OPL) , Volume 375: Symposia AA – Applications of Synchrotron Radiation Techniques to Materials Science , 1994 , 105
Copyright
Copyright © Materials Research Society 1995

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