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Oxide interfaces with enhanced ion conductivity

Published online by Cambridge University Press:  17 December 2013

Carlos Leon ,
Jacobo Santamaria  and
Bernard A. Boukamp
Carlos Leon
Affiliation:
Department of Applied Physics, Universidad Complutense, Madrid;[email protected]
Jacobo Santamaria
Affiliation:
Applied Physics Department, Universidad Complutense, Madrid;[email protected]
Bernard A. Boukamp
Affiliation:
University of Twente, The Netherlands;[email protected]
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Abstract

The new field of nano-ionics is expected to yield large improvements in the performance of oxide-based energy generation and storage devices based on exploiting size effects in ion conducting materials. The search for novel materials with enhanced ionic conductivity for application in energy devices has uncovered an exciting new facet of oxide interfaces. With judicious choice of the constituent materials, oxide heterostructures can exhibit enhanced ion mobility compared to the bulk counterparts. Here we review recent experimental and theoretical progress on enhancement of oxide-ion conductivity arising in oxide ultrathin layers and at their interfaces, and describe the different scenarios, space-charge effects, epitaxial strain, and atomic reconstruction at the interface, proposed to account for the observed conductivity enhancement.

Keywords

Ionic conductornanoscaleoxidethin film
Type
Functional Oxide Interfaces
Information
MRS Bulletin , Volume 38 , Issue 12: Functional Oxide Interfaces , December 2013 , pp. 1056 - 1063
Copyright
Copyright © Materials Research Society 2013 

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