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Plasmonic excitation and manipulation with an electron beam

Published online by Cambridge University Press:  15 August 2012

Ernst Jan R. Vesseur ,
Javier Aizpurua ,
Toon Coenen ,
Alejandro Reyes-Coronado ,
Philip E. Batson  and
Albert Polman
Ernst Jan R. Vesseur
Affiliation:
Caelux Corporation, Pasadena, CA; [email protected]
Javier Aizpurua
Affiliation:
Center for Materials Physics of the Spanish National Council for Scientific Research CSIC and DIPC, San Sebastian, Spain; [email protected]
Toon Coenen
Affiliation:
FOM Institute AMOLF, Amsterdam, The Netherlands; [email protected]
Alejandro Reyes-Coronado
Affiliation:
Institute of Physics, Autonomous University of Puebla, Mexico; [email protected]
Philip E. Batson
Affiliation:
Institute for Advanced Materials, Devices and Nanotechnology, Rutgers University; [email protected]
Albert Polman
Affiliation:
FOM Institute AMOLF, Amsterdam, The Netherlands; [email protected]
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Abstract

When an electron beam passes through or near a metal structure, it will excite surface plasmons, providing a unique way to access surface plasmon behavior at the nanoscale. An electron beam focused to nanometer dimensions thus functions as a point source that is able to probe the local plasmonic mode structure at deep-subwavelength resolution. In this article, we show how well-controlled coupling between an electron beam and surface plasmons, combined with a far-field detection system, allows characterization and manipulation of plasmons on a variety of plasmonic devices. By mapping the spatial profile of inelastic scattering to resonant modes, the dispersion and losses of surface plasmons are resolved. The technique further allows probing of the confinement of plasmons within cavities and measuring the angular emission profile of nanoantennas. The coupling of electrons to surface plasmons allows the use of the electron beam as a dipole emitter that can be positioned at will. The beam position thereby can select between modes with different symmetries. This effect can be used to exert forces on plasmonic structures on the nanometer length scale with great control.

Keywords

Optical propertieselectron irradiationSEMSTEMmetal
Type
Research Article
Information
MRS Bulletin , Volume 37 , Issue 8: Plasmonics , August 2012 , pp. 752 - 760
Copyright
Copyright © Materials Research Society 2012

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