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Inkjet-Printing of Methylammonium Lead Trihalide Perovskite as Active Layers for Optoelectronic Devices

Published online by Cambridge University Press:  12 February 2018

Charles Trudeau ,
Martin Bolduc ,
Patrick Beaupré ,
Jaime Benavides-Guerrero ,
Bruno Tremblay  and
Sylvain G. Cloutier
Charles Trudeau*
Affiliation:
Institut National d’Optique, 2740Einstein Street, Québec, QC, Canada G1P 4S4 Department of Electrical Engineering, École de Technologie Supérieure, 1100Notre-Dame Ouest, Montréal, QC, Canada H3C 1K3
Martin Bolduc
Affiliation:
Institut National d’Optique, 2740Einstein Street, Québec, QC, Canada G1P 4S4
Patrick Beaupré
Affiliation:
Institut National d’Optique, 2740Einstein Street, Québec, QC, Canada G1P 4S4
Jaime Benavides-Guerrero
Affiliation:
Department of Electrical Engineering, École de Technologie Supérieure, 1100Notre-Dame Ouest, Montréal, QC, Canada H3C 1K3
Bruno Tremblay
Affiliation:
Institut National d’Optique, 2740Einstein Street, Québec, QC, Canada G1P 4S4
Sylvain G. Cloutier
Affiliation:
Department of Electrical Engineering, École de Technologie Supérieure, 1100Notre-Dame Ouest, Montréal, QC, Canada H3C 1K3
*
*(Email: [email protected])
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Abstract

New routes in additive devices fabrication techniques and advances in printable materials are required to meet the ever increasing demands for low-cost and large-area flexible electronics. In particular, perovskite-based materials have gained an appeal due to their unique optoelectronics and ferroelectrics properties, which may replace p-n junction in semiconductor devices. Metal-organic methylammonium lead trihalide perovskite formulations have been extensively studied in the last few years as promising materials for use in printed electronics, which do not require high temperatures or vacuum environment, contrary to conventional semiconductor fabrication techniques. In this work, digital inkjet-printing in ambient atmosphere is proposed as a deposition pathway for the fabrication of perovskite active layers in photodetector and thin-film photovoltaic device architectures. The device architecture containing a printed perovskite active layer sandwiched between TiO2 and Spiro-OMeTAD as electron and hole transport layers, respectively, as well as layer-on-layer fabrication and responsivity spectra of the perovskite-based device are presented.

Keywords

ink-jet printingoptoelectronicthin film
Type
Articles
Information
MRS Advances , Volume 3 , Issue 32: Energy and Sustainability , 2018 , pp. 1837 - 1842
Copyright
Copyright © Materials Research Society 2018 

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References

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