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Trajectories, diffusion, and interactions of single ceria particles on a glass surface observed by evanescent wave microscopy

Published online by Cambridge University Press:  27 January 2020

Jihoon Seo Open the ORCID record for Jihoon Seo [Opens in a new window] ,
Akshay Gowda ,
Panart Khajornrungruang ,
Satomi Hamada ,
Taeseup Song  and
Suryadevara Babu Open the ORCID record for Suryadevara Babu [Opens in a new window]
Jihoon Seo*
Affiliation:
Department of Chemical and Biomolecular Engineering, Clarkson University, Potsdam, New York 13699, USA; and Center for Advanced Materials Processing, Clarkson University, Potsdam, New York 13699, USA
Akshay Gowda
Affiliation:
Department of Chemical and Biomolecular Engineering, Clarkson University, Potsdam, New York 13699, USA
Panart Khajornrungruang
Affiliation:
Department of Mechanical Information Science and Technology, Kyushu Institute of Technology, Iizuka-shi, Fukuoka-ken 820-8502, Japan
Satomi Hamada
Affiliation:
Advanced Technology Division, EBARA Corporation, Fujisawa-shi, Kanagawa 251-8502, Japan
Taeseup Song
Affiliation:
Department of Energy Engineering, Hanyang University, Seoul 04763, South Korea
Suryadevara Babu*
Affiliation:
Department of Chemical and Biomolecular Engineering, Clarkson University, Potsdam, New York 13699, USA; and Center for Advanced Materials Processing, Clarkson University, Potsdam, New York 13699, USA
*
a)Address all correspondence to these authors. e-mail: [email protected]
b)e-mail: [email protected]
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Abstract

Using evanescent wave (EW)–based optical detection methods coupled with video microscopy, we investigated in situ trajectories, diffusion, and interaction energies of ∼140 nm ceria particles near a glass surface at pH 3, 5, and 7. Trajectories of a single ceria particle in a 2D (x–y) plane were obtained by linking its time-sequenced positions. Diffusion coefficients of several single ceria particles were calculated from their respective mean-square displacement (MSD) versus time curves, and the results were interpreted based on the interaction potential energy curves obtained from Boltzmann statistics of the EW scattering intensity fluctuations of the particles. The types and characteristics of particle motions were determined by analyzing the MSD curves. Whereas both confined or subdiffusive and Brownian motions of the particles were observed at pH 7, only confined motion was seen at pH 3 and 5, and their corresponding diffusion coefficients are similar to those reported by several authors.

Keywords

colloidsurface reactionadsorption
Type
Article
Information
Journal of Materials Research , Volume 35 , Issue 3 , 14 February 2020 , pp. 321 - 331
Copyright
Copyright © Materials Research Society 2020

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Footnotes

c)

These authors contributed equally to this work.

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