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Effect of electropulsing-ultrasonic surface treatment on the surface properties and the corrosion behavior of 45 steel

Published online by Cambridge University Press:  16 May 2016

Bing Zhang ,
Haibo Wang ,
Shuo Zhang ,
Guolin Song ,
Song-Zhu Kure-Chu ,
Xinglong Wang ,
Jie Kuang  and
Guoyi Tang
Bing Zhang
Affiliation:
Advanced Materials Institute, Graduate School at Shenzhen, Tsinghua University, Shenzhen 518055, People's Republic of China
Haibo Wang
Affiliation:
Advanced Materials Institute, Graduate School at Shenzhen, Tsinghua University, Shenzhen 518055, People's Republic of China; and Key Laboratory for Advanced Materials of Ministry of Education, Department of Materials Science and Engineering, Tsinghua University, Beijing 100084, People's Republic of China
Shuo Zhang
Affiliation:
Advanced Materials Institute, Graduate School at Shenzhen, Tsinghua University, Shenzhen 518055, People's Republic of China
Guolin Song
Affiliation:
Advanced Materials Institute, Graduate School at Shenzhen, Tsinghua University, Shenzhen 518055, People's Republic of China
Song-Zhu Kure-Chu
Affiliation:
Department of Chemistry and Bioengineering, Faculty of Engineering, Iwate University, Iwate 020-8551, Japan
Xinglong Wang
Affiliation:
Shenzhen Pingjin Corporation, Shenzhen 518100, People's Republic of China
Jie Kuang
Affiliation:
Advanced Materials Institute, Graduate School at Shenzhen, Tsinghua University, Shenzhen 518055, People's Republic of China; and Key Laboratory for Advanced Materials of Ministry of Education, Department of Materials Science and Engineering, Tsinghua University, Beijing 100084, People's Republic of China
Guoyi Tang*
Affiliation:
Advanced Materials Institute, Graduate School at Shenzhen, Tsinghua University, Shenzhen 518055, People's Republic of China; and Key Laboratory for Advanced Materials of Ministry of Education, Department of Materials Science and Engineering, Tsinghua University, Beijing 100084, People's Republic of China
*
a) Address all correspondence to this author. e-mail: [email protected]
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Abstract

In the present study, the surface properties and the corrosion behavior of a nanocrystalline surface layer fabricated on 45 steel by electropulsing-ultrasonic surface treatment (EUST) were investigated. EUST offered the specimen a smooth (R a < 0.33 µm) surface layer with nanoscale grains and compressive stress by the synergistic effect of high-energy electropulsing processing and ultrasonic impact. Open-circuit potential, potentiodynamic polarization, and electrochemical impedance spectroscopy studies indicated that EUST-induced surface nanocrystallization decreased the corrosion susceptibility of 45 steel in 3.5 wt% NaCl aqueous solution, leading to a decrease in corrosion current density (i corr) by 55% and an increase in charge transfer resistance (R ct) by 36%. The enhancement in surface comprehensive mechanical properties and corrosion resistance can be explained in terms of the decrease in surface roughness, the extent of grain refinement and the change of stress state, which were closely related to the introduction of high-energy electropulsing processing.

Keywords

microstructurenanoscalecorrosion
Type
Articles
Information
Journal of Materials Research , Volume 31 , Issue 14 , 28 July 2016 , pp. 2114 - 2124
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Copyright
Copyright © Materials Research Society 2016 

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Footnotes

Contributing Editor: Jürgen Eckert

References

REFERENCES

Dai, K., Villegas, J., Stone, Z., and Shaw, L.: Finite element modeling of the surface roughness of 5052 Al alloy subjected to a surface severe plastic deformation process. Acta Mater. 52(20), 5771 (2004).Google Scholar
Murashkin, M.Y., Sabirov, I., Kazykhanov, V.U., Bobruk, E.V., Dubravina, A.A., and Valiev, R.Z.: Enhanced mechanical properties and electrical conductivity in ultrafine-grained Al alloy processed via ECAP-PC. J. Mater. Sci. 48, 4501 (2013).Google Scholar
Yin, F., Hu, S., Hua, L., Wang, X., Suslov, S., and Han, Q.: Surface nanocrystallization and numerical modeling of low carbon steel by means of ultrasonic shot peening. Metall. Mater. Trans. A 46(3), 1253 (2015).Google Scholar
Lu, K. and Lu, J.: Nanostructured surface layer on metallic materials induced by surface mechanical attrition treatment. Mater. Sci. Eng., A 375–377, 38 (2004).CrossRefGoogle Scholar
Ya, M., Xing, Y., Dai, F., Lu, K., and Lu, J.: Study of residual stress in surface nanostructured AISI 316L stainless steel using two mechanical methods. Surf. Coat. Technol. 168(2), 148 (2003).Google Scholar
Yanbin, J., Guoyi, T., Lei, G., Shaonan, W., Zhuohui, X., Chanhung, S., and Yaohua, Z.: Effect of electropulsing treatment on solid solution behavior of an aged Mg alloy AZ61 strip. J. Mater. Res. 23(10), 2685 (2008).Google Scholar
Guan, L., Tang, G.Y., Chu, P.K., and Jiang, Y.B.: Enhancement of ductility in Mg–3Al–1Zn alloy with tilted basal texture by electropulsing. J. Mater. Res. 24(12), 3674 (2009).Google Scholar
Hamal, D.B. and Klabunde, K.J.: Valence state and catalytic role of cobalt ions in cobalt TiO2 nanoparticle photocatalysts for acetaldehyde degradation under visible light. J. Phys. Chem. C 115(35), 17359 (2011).Google Scholar
Tao, N.R., Wang, Z.B., Tong, W.P., Sui, M.L., Lu, J., and Lu, K.: An investigation of surface nanocrystallization mechanism in Fe induced by surface mechanical attrition treatment. Acta Mater. 50(18), 4603 (2002).CrossRefGoogle Scholar
Han, H., Gao, Y., Zhang, Y., Du, S., and Liu, H.: Effect of magnetic field distribution of friction surface on friction and wear properties of 45 steel in DC magnetic field. Wear 328–329, 422 (2015).Google Scholar
Oguzie, E.E., Li, Y., and Wang, F.: Effect of surface nanocrystallization on corrosion and corrosion inhibition of low carbon steel: Synergistic effect of methionine and iodide ion. Electrochim. Acta 52(24), 6988 (2007).Google Scholar
Laleh, M. and Kargar, F.: Effect of surface nanocrystallization on the microstructural and corrosion characteristics of AZ91D magnesium alloy. J. Alloys Compd. 509(37), 9150 (2011).CrossRefGoogle Scholar
Oguzie, E.E., Wang, S.G., Li, Y., and Wang, F.H.: Corrosion and corrosion inhibition characteristics of bulk nanocrystalline ingot iron in sulphuric acid. J. Solid State Electrochem. 12(6), 721 (2008).Google Scholar
Jelliti, S., Richard, C., Retraint, D., Roland, T., Chemkhi, M., and Demangel, C.: Effect of surface nanocrystallization on the corrosion behavior of Ti–6Al–4V titanium alloy. Surf. Coat. Technol. 224, 82 (2013).CrossRefGoogle Scholar
Yang, J.X., Cui, F.Z., Lee, I-S., Zhang, Y., Yin, Q.S., Xia, H., and Yang, S.X.: In vivo biocompatibility and degradation behavior of Mg alloy coated by calcium phosphate in a rabbit model. J. Biomater. Appl. 27(2), 153 (2011).Google Scholar
Yanbin, J., Guoyi, T., Chanhung, S., Yaohua, Z., Lei, G., Shaonan, W., and Zhuohui, X.: Improved ductility of aged Mg–9Al–1Zn alloy strip by electropulsing treatment. J. Mater. Res. 24(5), 1810 (2009).Google Scholar
Ye, X., Tang, G., Song, G., and Kuang, J.: Effect of electropulsing treatment on the microstructure, texture, and mechanical properties of cold-rolled Ti–6Al–4V alloy. J. Mater. Res. 29(14), 1500 (2014).Google Scholar
Rahnama, A. and Qin, R.S.: The effect of electropulsing on the interlamellar spacing and mechanical properties of a hot-rolled 0.14% carbon steel. Mater. Sci. Eng., A 627, 145 (2015).CrossRefGoogle Scholar
Lu, W.J., Zhang, X.F., and Qin, R.S.: Electropulsing-induced strengthening of steel at high temperature. Philos. Mag. Lett. 94(11), 688 (2014).Google Scholar
Kuang, J., Li, X., Ye, X., Tang, J., Liu, H., Wang, J., and Tang, G.: Microstructure and texture evolution of magnesium alloys during electropulse treatment. Metall. Mater. Trans. A 46(4), 1789 (2015).Google Scholar
Ye, X., Liu, T., Ye, Y., Wang, H., Tang, G., and Song, G.: Enhanced grain refinement and microhardness of Ti–Al–V alloy by electropulsing ultrasonic shock. J. Alloys Compd. 621, 66 (2015).CrossRefGoogle Scholar
Ye, X., Kuang, J., Li, X., and Tang, G.: Microstructure, properties and temperature evolution of electro-pulsing treated functionally graded Ti–6Al–4V alloy strip. J. Alloys Compd. 599, 1 (2014).CrossRefGoogle Scholar
Maawad, E., Brokmeier, H-G., Wagner, L., Sano, Y., and Genzel, C.: Investigation on the surface and near-surface characteristics of Ti–2.5Cu after various mechanical surface treatments. Surf. Coat. Technol. 205(12), 3644 (2011).Google Scholar
Ye, X., Yang, Y., and Tang, G.: Microhardness and corrosion behavior of surface gradient oxide coating on the titanium alloy strips under high energy electro-pulsing treatment. Surf. Coat. Technol. 258, 467 (2014).CrossRefGoogle Scholar
Ye, X., Tse, Z.T.H., Tang, G., and Song, G.: The effect of electropulsing induced gradient topographic oxide coating of Ti–Al–V alloy strips on the fibroblast adhesion and growth. Surf. Coat. Technol. 261, 213 (2015).Google Scholar
Ye, X., Wang, L., Tse, Z.T.H., Tang, G., and Song, G.: Effects of high-energy electro-pulsing treatment on microstructure, mechanical properties and corrosion behavior of Ti–6Al–4V alloy. Mater. Sci. Eng., C 49, 851 (2015).Google Scholar
Balusamy, T., Kumar, S., and Sankara Narayanan, T.S.N.: Effect of surface nanocrystallization on the corrosion behavior of AISI 409 stainless steel. Corros. Sci. 52(11), 3826 (2010).Google Scholar
Kumar, S. and Sankara Narayanan, T.S.N.: Corrosion behavior of Ti–15Mo alloy for dental implant applications. J. Dent. 36(7), 500 (2008).CrossRefGoogle ScholarPubMed
Ye, X., Li, X., Song, G., and Tang, G.: Effect of recovering damage and improving microstructure in the titanium alloy strip under high-energy electropulses. J. Alloys Compd. 616, 173 (2014).Google Scholar
Zhou, Y., Zhang, W., Wang, B., He, G., and Guo, J.: Grain refinement and formation of ultrafine-grained microstructure in a low-carbon steel under electropulsing. J. Mater. Res. 17(08), 2105 (2002).Google Scholar
Ye, X., Yang, Y., Song, G., and Tang, G.: Enhancement of ductility, weakening of anisotropy behavior and local recrystallization in cold-rolled Ti–6Al–4V alloy strips by high-density electropulsing treatment. Appl. Phys. A: Mater. Sci. Process. 117(4), 2251 (2014).Google Scholar
Wang, F., Huo, D., Li, S., and Fan, Q.: Inducing TiAl3 in titanium alloys by electric pulse heat treatment improves mechanical properties. J. Alloys Compd. 550, 133 (2013).Google Scholar
Ouici, H.B., Benali, O., Harek, Y., Larabi, L., Hammouti, B., and Guendouzi, A.: The effect of some triazole derivatives as inhibitors for the corrosion of mild steel in 5% hydrochloric acid. Res. Chem. Intermed. 39(7), 3089 (2013).Google Scholar
Bılgıç, S. and Çalıskan, N.: The effect of N-(1-toluidine) salicylaldimine on the corrosion of austenitic chromium–nickel steel. Appl. Surf. Sci. 152(1), 107 (1999).Google Scholar
Arslan, E., Totik, Y., Demirci, E., and Alsaran, A.: Influence of surface roughness on corrosion and tribological behavior of CP-Ti after thermal oxidation treatment. J. Mater. Eng. Perform. 19(3), 428 (2010).CrossRefGoogle Scholar
Yin, S., Li, D.Y., and Bouchard, R.: Effects of strain rate of prior deformation on corrosion and corrosive wear of AISI 1045 steel in a 3.5 Pct NaCl solution. Metall. Mater. Trans. A 38(5), 1032 (2007).Google Scholar
Hassani, S., Raeissi, K., Azzi, M., Li, D., Golozar, M.A., and Szpunar, J.A.: Improving the corrosion and tribocorrosion resistance of Ni–Co nanocrystalline coatings in NaOH solution. Corros. Sci. 51(10), 2371 (2009).Google Scholar
Srinivasan, P.B., Zettler, R., Blawert, C., and Dietzel, W.: Stress corrosion cracking of AZ61 magnesium alloy friction stir weldments in ASTM D1384 solution. Corros. Eng., Sci. Technol. 44, 477 (2009).Google Scholar
LÓpez, D.A., Simison, S.N., and de Sànchez, S.R.: The influence of steel microstructure on CO2 corrosion. EIS studies on the inhibition efficiency of benzimidazole. Electrochim. Acta 48(7), 845 (2003).Google Scholar
Lebrini, M., Bentiss, F., Vezin, H., and Lagrenée, M.: The inhibition of mild steel corrosion in acidic solutions by 2,5-bis(4-pyridyl)-1,3,4-thiadiazole: Structure-activity correlation. Corros. Sci. 48(5), 1279 (2006).CrossRefGoogle Scholar