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Nonlinear electrohydrodynamics of slightly deformed oblate drops

Published online by Cambridge University Press:  05 June 2015

Javier A. Lanauze
Affiliation:
Department of Chemical Engineering, Carnegie Mellon University, Pittsburgh, PA 15213, USA
Lynn M. Walker
Affiliation:
Department of Chemical Engineering, Carnegie Mellon University, Pittsburgh, PA 15213, USA
Aditya S. Khair*
Affiliation:
Department of Chemical Engineering, Carnegie Mellon University, Pittsburgh, PA 15213, USA
*
Email address for correspondence: [email protected]

Abstract

The transient deformation of a weakly conducting (‘leaky dielectric’) drop under a uniform DC electric field is computed via an axisymmetric boundary integral method, which accounts for surface charge convection and a finite relaxation time scale over which the drop interface charges. We focus on drops that attain an ultimate oblate (major axis normal to the applied field) steady-state configuration. The computations predict that as the time scale for interfacial charging increases, a shape transition from prolate deformation (major axis parallel to the applied field) to oblate deformation occurs at intermediate times due to the slow buildup of charge at the surface of the drop. Convection of surface charge towards the equator of the drop is shown to weaken the steady-state oblate deformation. Additionally, convection results in sharp shock-like variations in surface charge density near the equator of the drop. Our numerical results are then compared with an experimental system consisting of a millimetre-sized silicone oil drop suspended in castor oil. Agreement in the transient deformation is observed between our numerical results and experimental measurements for moderate electric field strengths. This suggests that both charge relaxation and charge convection are required, in general, to quantify the time-dependent deformation of leaky dielectric drops. Importantly, accurate prediction of the observed modest deformation requires a nonlinear model. Discrepancies between our numerical calculations and experimental results arise as the field strength is increased. We believe that this is due to the observed onset of rotation and three-dimensional flow at such high electric fields in the experiments, which an axisymmetric boundary integral formulation naturally cannot capture.

Type
Papers
Copyright
© 2015 Cambridge University Press 

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References

Ajayi, O. O. 1978 A note on Taylor’s electrohydrodynamic theory. Proc. R. Soc. Lond. A 364, 499507.Google Scholar
Allan, R. S. & Mason, S. G. 1962 Particle behaviour in shear and electric fields. I. Deformation and burst of fluid drops. Proc. R. Soc. Lond. A 267, 4561.Google Scholar
Baygents, J. C., Rivette, N. J. & Stone, H. A. 1998 Electrohydrodynamic deformation and interaction of drop pairs. J. Fluid Mech. 368, 359375.CrossRefGoogle Scholar
Collins, R. T., Sambath, K., Harris, M. T. & Basaran, O. A. 2013 Universal scaling laws for the disintegration of electrified drops. Proc. Natl Acad. Sci. USA 110, 49054910.Google Scholar
Esmaeeli, A. & Sharifi, P. 2011 Transient electrohydrodynamics of a liquid drop. Phys. Rev. E 84, 036308.CrossRefGoogle ScholarPubMed
Feng, J. Q. 1999 Electrohydrodynamic behaviour of a drop subjected to a steady uniform electric field at finite electric Reynolds number. Proc. R. Soc. Lond. A 455, 22452269.CrossRefGoogle Scholar
Feng, J. Q. & Scott, T. C. 1996 A computational analysis of electrohydrodynamics of a leaky dielectric drop in an electric field. J. Fluid Mech. 311, 289326.Google Scholar
Fernández, A. 2013 Modeling of electroconvective effects on the interaction between electric fields and low conductive drops. In ASME 2013 Fluids Engineering Division Summer Meeting, pp. V01CT25A004V01CT25A004. American Society of Mechanical Engineers.Google Scholar
Ha, J.-W. & Yang, S.-M. 2000a Deformation and breakup of Newtonian and non-Newtonian conducting drops in an electric field. J. Fluid Mech. 405, 131156.CrossRefGoogle Scholar
Ha, J.-W. & Yang, S.-M. 2000b Electrohydrodynamics and electrorotation of a drop with fluid less conductive than that of the ambient fluid. Phys. Fluids 12, 764772.Google Scholar
Halim, M. A. & Esmaeeli, A. 2013 Computational studies on the transient electrohydrodynamics of a liquid drop. Fluid Dyn. Mater. Process. 9, 435460.Google Scholar
Jones, T. B. 1984 Quincke rotation of spheres. IEEE Trans. Ind. Applics. 845849.Google Scholar
Lac, E. & Homsy, G. M. 2007 Axisymmetric deformation and stability of a viscous drop in a steady electric field. J. Fluid Mech. 590, 239264.CrossRefGoogle Scholar
Lanauze, J. A., Walker, L. M. & Khair, A. S. 2013 The influence of inertia and charge relaxation on electrohydrodynamic drop deformation. Phys. Fluids 25, 112101.CrossRefGoogle Scholar
Melcher, J. R. & Taylor, G. I. 1969 Electrohydrodynamics: a review of the role of interfacial shear stresses. Annu. Rev. Fluid Mech. 1, 111146.CrossRefGoogle Scholar
O’Konski, C. T. & Thacher, H. C. Jr. 1953 The distortion of aerosol droplets by an electric field. J. Phys. Chem. 57, 955958.CrossRefGoogle Scholar
Pozrikidis, C. 1992 Boundary Integral and Singularity Methods for Linearized Viscous Flow. Cambridge University Press.CrossRefGoogle Scholar
Pozrikidis, C. 2010 A Practical Guide to Boundary Element Methods with the Software Library BEMLIB. CRC Press.Google Scholar
Quincke, G. 1896 Ueber Rotationen im constanten electrischen Felde. Ann. Phys. 295, 417486.CrossRefGoogle Scholar
Salipante, P. F. & Vlahovska, P. M. 2010 Electrohydrodynamics of drops in strong uniform dc electric fields. Phys. Fluids 22, 112110.CrossRefGoogle Scholar
Saville, D. A. 1971 Electrohydrodynamic stability: effects of charge relaxation at the interface of a liquid jet. J. Fluid Mech. 48, 815827.Google Scholar
Saville, D. A. 1997 Electrohydrodynamics: the Taylor–Melcher leaky dielectric model. Annu. Rev. Fluid Mech. 29, 2764.Google Scholar
Sherwood, J. D. 1988 Breakup of fluid droplets in electric and magnetic fields. J. Fluid Mech. 188, 133146.Google Scholar
Stone, H. A., Lister, J. R. & Brenner, M. P. 1999 Drops with conical ends in electric and magnetic fields. Proc. R. Soc. Lond. A 455, 329347.Google Scholar
Supeene, G., Koch, C. R. & Bhattacharjee, S. 2008 Deformation of a droplet in an electric field: nonlinear transient response in perfect and leaky dielectric media. J. Colloid Interface Sci. 318, 463476.Google Scholar
Taylor, G. I. 1966 Studies in electrohydrodynamics. I. The circulation produced in a drop by electrical field. Proc. R. Soc. Lond. A 291, 159166.Google Scholar
Torza, S., Cox, R. G. & Mason, S. G. 1971 Electrohydrodynamic deformation and burst of liquid drops. Phil. Trans. R. Soc. Lond. A 269, 295319.Google Scholar
Tsukada, T., Katayama, T., Ito, Y. & Hozawa, M. 1993 Theoretical and experimental studies of circulations inside and outside a deformed drop under a uniform electric field. J. Chem. Engng Japan 26, 698703.Google Scholar
Vizika, O. & Saville, D. A. 1992 The electrohydrodynamic deformation of drops suspended in liquids in steady and oscillatory electric fields. J. Fluid Mech. 239, 121.Google Scholar
Wang, Z., Dong, Q., Zhang, Y., Wang, J. & Wen, J. 2014 Numerical study on deformation and interior flow of a droplet suspended in viscous liquid under steady electric fields. Adv. Mech. Engng 2014, 112.Google Scholar
Yezer, B. A., Khair, A. S., Sides, P. J. & Prieve, D. C. 2014 Use of electrochemical impedance spectroscopy to determine double-layer capacitance in doped nonpolar liquids. J. Colloid Interface Sci. 449, 212.CrossRefGoogle ScholarPubMed
Zhang, J., Zahn, J. D. & Lin, H. 2013 Transient solution for droplet deformation under electric fields. Phys. Rev. E 87, 043008.Google Scholar