Detailed geological mapping and geochemical analysis of early Palaeozoic granitoid plutons and dykes from the Taylor Valley and Ferrar Glacier region in south Victoria Land reveal two distinct suites. This suite subdivision-approach is a departure from previous lithology-based schemes and can be applied elsewhere in south Victoria Land. The older calc-alkaline Dry Valleys 1 suite is dominated by the compositionally variable Bonney Pluton, a flow-foliated concordant pluton with an inferred length of over 100 km. Plutons of this suite are elongate in a NW-SE direction and appear to have been subjected to major structural control during their emplacement. The younger alkali-calcic Dry Valleys 2 suite comprises discordant plutons and numerous dyke swarms with complex age relationships. Field characteristics of this suite indicate that it was passively emplaced into fractures at higher levels in the crust than the Dry Valleys 1 suite. Whole-rock geochemistry confirms this suite subdivision based on field relationships and indicates that the two suites were derived from different parent magmas by fractional crystallization. The Dry Valleys 1 suite resembles Cordilleran I-type granitoids and is inferred to be derived from partial melting of the upper mantle and/or lower crust above an ancient subduction zone. The Dry Valleys 2 suite resembles Caledonian I-type granitoids and may have resulted from a later episode of crustal extension.