The linear angular dispersion of a self-diffraction (SD) pulse, from a femtosecond laser pulse cleaning device, is compensated for by the use of a single prism. More than $500~\unicode[STIX]{x03BC}\text{J}$ first-order SD pulse has a contrast of $10^{12}$, which is about five orders of magnitude improvement from the input fundamental pulse. The wings of the distribution away from the main pulse in $\pm 1$ ps are cleaned with a contrast improvement of about $10^{7}$, which verifies the pulse cleaning ability of the SD process.

FERMI, the seeded free electron laser (FEL) in operation in Italy, is providing the User Community with unique fully coherent radiation, in the wavelength range 100–4 nm. FERMI is the first FEL fully synchronized by means of optical fibers. The optical timing system ensures an ultra-stable phase reference to its distributed clients. Several femtosecond longitudinal diagnostics verify the achieved performance; the bunch length monitor (BLM) and the bunch arrival monitor (BAM) will be presented in this paper. Feedback systems play a crucial role to guarantee the needed long-term electron beam stability. A real-time infrastructure allows shot-to-shot communication between front-end computers and the servers. Orbit feedbacks are useful in machine tuning, whereas longitudinal feedbacks control electron energy, compression and arrival time. A flexible software framework allows a rapid implementation of heterogeneous multi-input–multi-output (MIMO) longitudinal loops simply by selecting the appropriate sensors and actuators.

The interaction of Ti:sapphire laser, operating at high repetition rate of 75 MHz, with nickel-based super-alloy Inconel 600 was studied. The laser was emitting at 800 nm and ultrashort pulse duration was 160 fs. Nickel-based super-alloy surface modification was studied in a low laser energy/fluence regime of maximum 20 nJ–15 mJ/cm2, for short (10 s) and long irradiation times (range of minutes). Surface damage threshold of this material was estimated to be 1.46 nJ, i.e., 0.001 J/cm2 in air. The radiation absorbed from Ti:sapphire laser beam under these conditions generates at the surface a series of effects, such as direct material vaporization, plasma creation, formation of nano-structures and their larger aggregates, damage accumulation, etc. Laser induced surface morphological changes observed on Inconel 600 were: (1) intensive removal of surface material with crater like features; (2) material deposition at near and farther periphery and creation of nano-aggregates/nano-structures; (3) sporadic micro-cracking of the inner and outer damage area. Generally, features created on nickel-based super-alloy surface by high repetition rate femtosecond pulses are characterized by low inner/outer damage diameter of less than 11 µm/30 µm and relatively large depth on the order of 150 µm, in both low (10 s) and high (minutes) irradiation time regimes.

We study the details of a gradual change in electron properties from those of a nearly-free-electron (NFE) metal to those of a strongly-coupled plasma, in ultrashort pulse energy deposition in solid metal targets. Time scales shorter than those of a target surface layer expansion are considered. Both the case of an optical laser (visible or near infrared wavelengths range) and of a free electron laser (vacuum ultraviolet or X-ray) are treated. The mechanisms responsible for the change in electron behavior are isochoric melting, lattice charge disordering, and electron mean free path reduction. We find that the transition from metal to plasma usually occurs via an intermediate stage of a charge-disordered solid (solid plasma), in which ions are at their lattice sites but the ionization stages of individual ions differ due to ionization from localized bound states. Charge disordered state formation is very rapid (typically, few femtoseconds or few tens of femtoseconds). Pathway to charge-disordered state differs in simple metals and in noble metals. Probabilities are derived for electron impact ionization and 3-body recombination of a bound ionic state in solid-density medium, applicable both in metal and in plasma regime. An evolution of energy coupling between electron and ion subsystems, from metallic electron-phonon (e-ph) to plasma electron-ion (e-i) coupling, is considered. Substantial increase in coupling parameter is expected as a result of charge disorder.

We investigated the optical properties of pure copper irradiated by a femtosecond laser pulse. Self-absorption of 50-fs laser pulses at 800 nm and 400 nm wavelengths (below and above the interband absorption threshold, respectively) is studied for peak laser intensities up to 1015 W/cm2. Theoretical description of laser interaction with copper target is developed, solving numerically the energy balance equations for electron and ion subsystems together with Maxwell equations for laser radiation field inside the target. The theory accounts for both intraband and interband absorption mechanisms. We treated in detail the changes in electron structure and distribution function with an increase in electron temperature, as well as the ensuing changes in thermodynamic properties, collision frequencies, optical and transport coefficients. Experimental work on self-absorption of femtosecond laser pulses in copper targets at 800 nm and 400 nm wavelengths is ongoing. Results for 800 nm wavelength are reported. Theory and experiment are in good agreement.

We give on overview of recent advances in collisionally pumped optical field-ionization soft X-ray lasers developed at LOA. Saturated amplification has been achieved on the 5d-5p transition in Xe8+ at 41.8 nm, and on the 4d-4p transition in Kr8+ at 32.8 nm. We demonstrate a significant increase of the energy output from the Xe8+ laser driven within two types of wave-guide. Finally, we present results of a pioneering work aimed to set up and characterize the first true soft X-ray laser chain.

This paper reports on a novel approach for producing high energy femtosecond pulses without external amplification. The so-called chirped-pulse oscillator (CPO) concept is based on an extended-cavity oscillator, operating at small net positive intracavity group delay dispersion (GDD), over a broad spectral range by the use of chirped multilayer mirrors. The resultant chirped picosecond pulses are compressed by a dispersive delay line external to the laser cavity. Utilizing this technique, sub-30 fs pulses with an energy exceeding 200 nJ at a repetition rate of 11 MHz were produced. The demonstrated peak power in excess of 5 MW is the highest ever achieved from a cw-pumped laser and is expected to be scaleable to tens of megawatts by increasing the pump power and/or decreasing the repetition rate. The demonstrated source allows micromachining of any materials under relaxed focusing conditions.