Here we report on a simple-to-implement and cost-effective approach for laser pulse contrast enhancement, based on the ${\chi}^{(3)}$ nonlinear self-focusing effect. An intentionally induced and gently controlled self-focusing in a thin glass transforms the time-dependent intensity into variation in beam divergence. Followed by a spatial discriminating filter, only the strongly focused fraction traverses the setup, at the expense of efficiency. A numerical model, accounting for the pulse and material parameters via a Gaussian ABCD matrix, provides an estimate for the instantaneous beam waist and transmission efficiency, which enables us to evaluate the resulting contrast enhancement. The estimated contrast enhancement spans between 0.5 and 2.5 orders of magnitude, in conjunction with approximately 25%–90% estimated efficiency, depending on the pulse parameters. In a preliminary experiment we demonstrated the effect with 10s-μJ sub GW regime with approximately 40$\%$ efficiency and a contrast improvement of more than or equal to 20 dB.

In strong-field physics experiments with ultraintense lasers, a single-shot cross-correlator (SSCC) is essential for fast optimization of the pulse contrast and meaningful comparison with theory for each pulse shot. To simultaneously characterize an ultrashort pulse and its long pedestal, the SSCC device must have both a high resolution and a large temporal window. However, the resolution and window in all kinds of single-shot measurement contradict each other in principle. Here we propose and demonstrate a novel SSCC device with two separate measurement channels: channel-1 for the large-window pedestal measurement has a moderate resolution but a large window, while channel-2 for the ultrashort pulse measurement has a small window but a high resolution; this allows the accurate characterization of the pulse contrast in a single shot. A two-channel SSCC device with a 200-fs resolution and 114-ps window has been developed and tested for its application in ultraintense lasers at 800 nm.

Pulse contrast is a crucial parameter of high peak-power lasers since the prepulse noise may disturb laser–plasma interactions. Contrast measurement is thus a prerequisite to tackle the contrast challenge in high peak-power lasers. This paper presents the progress review of single-shot cross-correlator (SSCC) for real-time contrast characterization. We begin with the key technologies that enable an SSCC to simultaneously possess high dynamic range ($10^{10}$), large temporal window (50–70 ps) and high fidelity. We also summarize the instrumentation of SSCC prototypes and their applications on five sets of petawatt laser facilities in China. Finally, we discuss how to extend contrast measurements from time domain to spatiotemporal domain. Real-time and high-dynamic-range contrast measurements, provided by SSCC, can not only characterize various complex noises in high peak-power lasers but also guide the system optimization.