Magnetic screening as a cost-effective and non-time-consuming approach has been successfully carried out in Marambio soils and seems to be a suitable method for contamination assessment in Antarctic areas. Ferromagnetic minerals are found in most samples, and magnetite-like carriers are especially dominant in samples collected near pollution sources. Lead and zinc are the main trace elements that have adversely impacted on some areas in this station, both are end products from different pollution sources derived from fuel combustion and residues, solid waste, paints, etc. The correlation results between magnetic and chemical variables show moderate relationships varying from 0.409 to 0.663; this fact supports the use of magnetic parameters, such as magnetic susceptibility and bivariate ratios, for pollution monitoring. The magnetic properties, heavy metal contents, and related maps of these soils can be considered as a reference in the area for future temporal and/or spatial work.