A multiresonance metasurface antenna is proposed which has wide bandwidth and low-profile. The characteristic mode theory is used to design antenna structure. Three ideal modes are obtained by adjusting the mode currents to optimize the radiation performance of the antenna. The characteristic mode analysis is used to model, analyze, and optimize the antenna, revealing the physical characteristics of the metasurface antenna. The slot is not only used as the feeding structure for exciting characteristic modes but also introduces a slot mode. Combining the slot mode with the metasurface modes, the bandwidth of the antenna is broadened. The antenna element has a relative bandwidth of 43.7%. To obtain higher gain, a 2 × 2 antenna array is proposed. The antenna array is simulated, fabricated, and measured. The results show that the relative bandwidth of the proposed metasurface antenna array is 31.6% with the gain of 12.3–15.8 dBi over the operating bandwidth.