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Tunable Microstructures in Entropy-Stabilized Oxide Thin Films Studied with Unsupervised Machine Learning Assisted Electron Microscopy

Published online by Cambridge University Press:  22 July 2022

Leixin Miao ,
George N. Kotsonis ,
Jon-Paul Maria  and
Nasim Alem
Leixin Miao
Affiliation:
Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA, USA
George N. Kotsonis
Affiliation:
Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA, USA
Jon-Paul Maria
Affiliation:
Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA, USA
Nasim Alem
Affiliation:
Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA, USA

Abstract

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Type
Advanced Imaging and Spectroscopy for Nanoscale Materials
Information
Microscopy and Microanalysis , Volume 28 , Supplement S1 , August 2022 , pp. 2594 - 2596
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Copyright
Copyright © Microscopy Society of America 2022

References

Rost, C.M., Sachet, E., Borman, T., Moballegh, A., Dickey, E.C., Hou, D., Jones, J.L., Curtarolo, S., Maria, J.P., Entropy-stabilized oxides, Nat. Commun. 6 (2015) 1–8. https://doi.org/10.1038/ncomms9485.CrossRefGoogle ScholarPubMed
Sarkar, A., Velasco, L., Wang, D., Wang, Q., Talasila, G., de Biasi, L., Kübel, C., Brezesinski, T., Bhattacharya, S.S., Hahn, H., Breitung, B., High entropy oxides for reversible energy storage, Nat. Commun. 9 (2018) 1–9. https://doi.org/10.1038/s41467-018-05774-5.CrossRefGoogle ScholarPubMed
Jiang, B., Yu, Y., Cui, J., Liu, X., Xie, L., Liao, J., Zhang, Q., Huang, Y., Ning, S., Jia, B., Zhu, B., Bai, S., Chen, L., Pennycook, S.J., He, J., High-entropy-stabilized chalcogenides with high thermoelectric performance, Science. 371 (2021) 830–834. https://doi.org/10.1126/science.abe1292.CrossRefGoogle ScholarPubMed
Li, T., Yao, Y., Huang, Z., Xie, P., Liu, Z., Yang, M., Gao, J., Zeng, K., Brozena, A.H., Pastel, G., Jiao, M., Dong, Q., Dai, J., Li, S., Zong, H., Chi, M., Luo, J., Mo, Y., Wang, G., Wang, C., Shahbazian-Yassar, R., Hu, L., Denary oxide nanoparticles as highly stable catalysts for methane combustion, Nat. Catal. 4 (2021) 62–70. https://doi.org/10.1038/s41929-020-00554-1.CrossRefGoogle Scholar
Cantor, B., Chang, I.T.H., Knight, P., Vincent, A.J.B., Microstructural development in equiatomic multicomponent alloys, Mater. Sci. Eng. A. 375–377 (2004) 213–218. https://doi.org/10.1016/j.msea.2003.10.257.CrossRefGoogle Scholar
Miao, L., Kotsonis, G., Ciston, J., Ophus, C., Maria, J.-P., Alem, N., Impact of the Synthesis Kinetics of Entropy-stabilized Oxide Thin Films Probed with 4D-STEM and STEM-EELS, Microsc. Microanal. 27 (2021) 352–354. https://doi.org/DOI:10.1017/S143192762100180X.CrossRefGoogle Scholar
Kotsonis, G.N., Meisenheimer, P.B., Miao, L., Roth, J., Wang, B., Shafer, P., Engel-Herbert, R., Alem, N., Heron, J.T., Rost, C.M., Maria, J.P., Property and cation valence engineering in entropy-stabilized oxide thin films, Phys. Rev. Mater. 4 (2020) 100401. https://doi.org/10.1103/PhysRevMaterials.4.100401.CrossRefGoogle Scholar
L.M., G.N.K, J.P.M., and N.A acknowledge the support by NSF through the Pennsylvania State University Materials Research Science and Engineering Center DMR 2011839. L.M and N.A. acknowledge the Air Force Office of Scientific Research (AFOSR) program FA9550-18-1-0277 as well as GAME MURI, 10059059-PENN for support. L.M. and N.A. appreciate the support and resources from NSF-MRSEC-sponsored Materials Characterization Lab (MCL) at Penn State.Google Scholar