Recent results in the development of diode-driven high energy, high repetition rate, picosecond lasers, including the demonstration of a cryogenic Yb:YAG active mirror amplifier that produces 1.5 J pulses at 500 Hz repetition rate (0.75 kW average power) are reviewed. These pulses are compressed resulting in the generation of ${\sim}5~\text{ps}$ duration, 1 J pulses with 0.5 kW average power. A full characterization of this high power cryogenic amplifier, including at-wavelength interferometry of the active region under ${>}1~\text{kW}$ average power pump conditions, is presented. An initial demonstration of operation at 1 kW average power (1 J, 1 kHz) is reported.

As our understanding of the environmental impact of fossil fuel based energy production increases, it is becoming clear that the world needs a new energy solution to meet the challenges of the future. A transformation is required in the energy market to meet the need for low carbon, sustainable, affordable generation matched with security of supply. In the short term, an increasing contribution from renewable sources may provide a solution in some locations. In the longer term, low carbon, sustainable solutions must be developed to meet base load energy demand, if the world is to avoid an ever increasing energy gap and the attendant political instabilities. Laser-driven inertial fusion energy (IFE) may offer such a solution.

A petawatt facility fully based on noncollinear optical parametric chirped pulse amplification (NOPCPA) technology, Vulcan OPPEL (Vulcan OPCPA PEtawatt Laser), is presented. This system will be coupled with the existing hybrid-CPA/OPCPA VULCAN laser system (500 J, 500 fs beamline; 250 J, ns regime beamline) based on Nd:glass amplification. Its pulse duration (20 times shorter) combined with the system design will allow the auxiliary beamline and its secondary sources to be used as probe beams for longer pulses and their interactions with targets. The newly designed system will be mainly dedicated to electron beam generation, but could also be used to perform a variety of particle acceleration and optical radiation detection experimental campaigns. In this communication, we present the entire beamline design discussing the technology choices and the design supported by extensive simulations for each system section. Finally, we present experimental results and details of our commissioned NOPCPA picosecond front end, delivering 1.5 mJ, ~180 nm (1/e2) of bandwidth compressed to sub-15 fs.

A 100-J-level Nd:glass laser system in nanosecond-scale pulse width has been constructed to perform as a standard source of high-fluence-laser science experiments. The laser system, operating with typical pulse durations of 3–5 ns and beam diameter 60 mm, employs a sequence of successive rod amplifiers to achieve 100-J-level energy at 1053 nm at 3 ns. The frequency conversion can provide energy of 50-J level at 351 nm. In addition to the high stability of the energy output, the most valuable of the laser system is the high spatiotemporal beam quality of the output, which contains the uniform square pulse waveform, the uniform flat-top spatial fluence distribution and the uniform flat-top wavefront.

In high power laser facility for inertial confinement fusion research, final optics assembly (FOA) plays a critical role in the frequency conversion, beam focusing, color separation, beam sampling and debris shielding. The design and performance of FOA in SG-II Upgrade laser facility are mainly introduced here. Due to the limited space and short focal length, a coaxial aspheric wedged focus lens is designed and applied in the FOA configuration. Then the ghost image analysis, the focus characteristic analysis, the B integral control design and the optomechanical design are carried out in the FOA design phase. In order to ensure the FOA performance, two key technologies are developed including measurement and adjustment technique of the wedged focus lens and the stray light management technique based on ground glass. Experimental results show that the design specifications including laser fluence, frequency conversion efficiency and perforation efficiency of the focus spot have been achieved, which meet the requirements of physical experiments well.

Various coatings in high-power laser facilities suffer from laser damage due to nodule defects. We propose a nodule dome removal (NDR) strategy to eliminate unwanted localized electric-field (E-field) enhancement caused by nodule defects, thereby improving the laser-induced damage threshold (LIDT) of laser coatings. It is theoretically demonstrated that the proposed NDR strategy can reduce the localized E-field enhancement of nodules in mirror coatings, polarizer coatings and beam splitter coatings. An ultraviolet (UV) mirror coating is experimentally demonstrated using the NDR strategy. The LIDT is improved to about 1.9 and 2.2 times for the UV mirror coating without artificial nodules and the UV mirror coating with artificial nodule seeds with a diameter of 1000 nm, respectively. The NDR strategy, applicable to coatings prepared by different deposition methods, improves the LIDT of laser coating without affecting other properties, such as the spectrum, stress and surface roughness, indicating its broad applicability in high-LIDT laser coatings.

We report on a target system supporting automated positioning of nano-targets with a precision resolution of $4~\unicode[STIX]{x03BC}\text{m}$ in three dimensions. It relies on a confocal distance sensor and a microscope. The system has been commissioned to position nanometer targets with 1 Hz repetition rate. Integrating our prototype into the table-top ATLAS 300 TW-laser system at the Laboratory for Extreme Photonics in Garching, we demonstrate the operation of a 0.5 Hz laser-driven proton source with a shot-to-shot variation of the maximum energy about 27% for a level of confidence of 0.95. The reason of laser shooting experiments operated at 0.5 Hz rather than 1 Hz is because the synchronization between the nano-foil target positioning system and the laser trigger needs to improve.

The status of the European X-ray Free-Electron Laser (European XFEL), under construction near Hamburg, Germany, is described. The start of operations of the LCLS at SLAC and of SACLA in Japan has already produced impressive scientific results. The European XFEL facility is powered by a 17.5 GeV superconducting linear accelerator that, compared to these two operating facilities, will generate two orders of magnitude more pulses per second, up to 27 000. It can therefore support modes of operation switching the beam up to 30 times per second among three different experiments, providing each of them with thousands of pulses per second. The scientific possibilities opened up by these capabilities are briefly described, together with the current instrumental developments (in optics, detectors, lasers, etc.) that are necessary to implement this program.

As an attractive collector medium for hypervelocity particles, combined with outstanding physical properties and suitable compositional characteristics, SiO2 aerogel has been deployed on outer space missions and laser shock-loaded collection experiments. In this paper, impact experiments were conducted to understand the penetration process of irregular grains, irregular Al2O3 grains with two different sizes and speeds (~110 μm@7 km/s, ~251 μ[email protected] km/s) at various density silica aerogels. By classifying the shapes of projectile residues and tracks, the morphology of tracks was analyzed. It was observed that there were several kinds of typical tracks in the penetration of irregular grains, accompanied by residues with the shapes of near-sphere, polyhedron, streamlined body wedge, and rotator. The rotational behavior was demonstrated by the final status of one flake projectile as direct evidence. In addition, there was no obvious relationship between the track length and experimental parameters, which may be caused by the uncertain interaction between aerogels and irregular particles. In addition, it confirmed the existence of fragmentation, melting situation by observing the shape of the impact entrance hole. At the same time, optical coherence tomography was used to observe the detail of tracks clearly, which provided a method to characterize the tracks nondestructively.

A new generation of high power laser facilities will provide laser pulses with extremely high powers of 10 petawatt (PW) and even 100 PW, capable of reaching intensities of $10^{23}~\text{W}/\text{cm}^{2}$ in the laser focus. These ultra-high intensities are nevertheless lower than the Schwinger intensity $I_{S}=2.3\times 10^{29}~\text{W}/\text{cm}^{2}$ at which the theory of quantum electrodynamics (QED) predicts that a large part of the energy of the laser photons will be transformed to hard Gamma-ray photons and even to matter, via electron–positron pair production. To enable the investigation of this physics at the intensities achievable with the next generation of high power laser facilities, an approach involving the interaction of two colliding PW laser pulses is being adopted. Theoretical simulations predict strong QED effects with colliding laser pulses of ${\geqslant}10~\text{PW}$ focused to intensities ${\geqslant}10^{22}~\text{W}/\text{cm}^{2}$.

High-power fiber lasers have experienced a dramatic development over the last decade. Further increasing the output power needs an upscaling of the fiber mode area, while maintaining a single-mode output. Here, we propose an all-solid anti-resonant fiber (ARF) structure, which ensures single-mode operation in broadband by resonantly coupling higher-order modes into the cladding. A series of fibers with core sizes ranging from 40 to 100 μm are proposed exhibiting maximum mode area exceeding 5000 μm2. Numerical simulations show this resonant coupling scheme provides a higher-order mode (mainly TE01, TM01, and HE21) suppression ratio of more than 20 dB, while keeping the fundamental mode loss lower than 1 dB/m. The proposed structure also exhibits high tolerance for core index depression.

An all-fiberized and narrow-bandwidth master oscillator power amplification (MOPA) system with record output power of 4 kW level and slope efficiency of 78% is demonstrated. Tandem pumping strategy is tentatively introduced into the narrow-bandwidth MOPA system for thermally induced mode instability (TMI) suppression. The stimulated Brillouin scattering (SBS) effect is balanced by simply using one-stage phase modulation technique. With different phase modulation signals, SBS limited output powers of 336 W, 1.2 kW and 3.94 kW are respectively achieved with spectral bandwidths accounting for 90% power of ${\sim}$0.025, 0.17 and ${\sim}$0.89 nm. Compared with our previous 976 nm pumping system, TMI threshold is overall boosted to be ${>}$5 times in which tandem pumping increases the TMI threshold of ${>}$3 times. The beam quality ($M^{2}$ factor) of the output laser is well within 1.5 below the TMI threshold while it is ultimately saturated to be 1.86 with the influence of TMI at maximal output power. Except for SBS and TMI, stimulated Raman scattering (SRS) effect will be another challenge for further power scaling. In such a high power MOPA system, multi-detrimental effects (SBS, SRS and TMI) will coexist and may be mutual-coupled, which could provide a well platform for further comprehensively investigating and optimizing the high power, narrow-bandwidth fiber amplifiers.

The quantum vacuum plays a central role in physics. Quantum electrodynamics (QED) predicts that the properties of the fermionic quantum vacuum can be probed by extremely large electromagnetic fields. The typical field amplitudes required correspond to the onset of the ‘optical breakdown’ of this vacuum, expected at light intensities >4.7×1029 W/cm2. Approaching this ‘Schwinger limit’ would enable testing of major but still unverified predictions of QED. Yet, the Schwinger limit is seven orders of magnitude above the present record in light intensity achieved by high-power lasers. To close this considerable gap, a promising paradigm consists of reflecting these laser beams off a mirror in relativistic motion, to induce a Doppler effect that compresses the light pulse in time down to the attosecond range and converts it to shorter wavelengths, which can then be focused much more tightly than the initial laser light. However, this faces a major experimental hurdle: how to generate such relativistic mirrors? In this article, we explain how this challenge could nowadays be tackled by using so-called ‘relativistic plasma mirrors’. We argue that approaching the Schwinger limit in the coming years by applying this scheme to the latest generation of petawatt-class lasers is a challenging but realistic objective.

We present a study of laser-driven ion acceleration with micrometre and sub-micrometre thick targets, which focuses on the enhancement of the maximum proton energy and the total number of accelerated particles at the PHELIX facility. Using laser pulses with a nanosecond temporal contrast of up to $10^{-12}$ and an intensity of the order of $10^{20}~\text{W}/\text{cm}^{2}$, proton energies up to 93 MeV are achieved. Additionally, the conversion efficiency at $45^{\circ }$ incidence angle was increased when changing the laser polarization to p, enabling similar proton energies and particle numbers as in the case of normal incidence and s-polarization, but reducing the debris on the last focusing optic.

Faraday effect measurements of holmium oxide (Ho2O3) ceramics-based magneto-optical materials, highly potential material candidates for high-energy laser Faraday isolators, are presented in this paper. Temperature dependence of the Verdet constant of nondoped Ho2O3 ceramics was measured for temperatures 15–305 K at $1.064~\unicode[STIX]{x03BC}\text{m}$ wavelength. The Verdet constant dispersion for wavelengths 0.5–$1~\unicode[STIX]{x03BC}\text{m}$ and $1.064~\unicode[STIX]{x03BC}\text{m}$ was measured for both nondoped Ho2O3 ceramics and Ho2O3 ceramics doped with terbium Tb3+ (0.2 at. %) and cerium Ce3+ (0.1 at. %) ions. The results suggest that the relatively low level of doping of Ho2O3 with these ions has no significant boosting impact on the Faraday effect. Therefore, other compositions of Ho2O3 ceramics-based magneto-optical materials, as well as various doping concentrations, should be further examined.

Over the past decade the integration of ultrafast spectroscopy with nanoscience has greatly propelled the development of nanoscience, as the key information gleaned from the mechanistic studies with the assistance of ultrafast spectroscopy enables a deeper understanding of the structure–function interplay and various interactions involved in the nanosystems. This mini-review presents an overview of the recent advances achieved in our ultrafast spectroscopy laboratory that address the ultrafast dynamics and related mechanisms in several representative nanomaterial complex systems by means of femtosecond time-resolved transient absorption spectroscopy. We attempt to convey instructive, consistent information regarding the important processes, pathways, dynamics, and interactions involved in the nanomaterial complex systems, most of which exhibit excellent performance in photocatalysis.

The quantum defect (QD) is an important issue that demands prompt attention in high-power fiber lasers. A large QD may aggravate the thermal load in the laser, which would impact the frequency, amplitude noise and mode stability, and threaten the security of the high-power laser system. Here, we propose and demonstrate a cladding-pumped Raman fiber laser (RFL) with QD of less than 1%. Using the Raman gain of the boson peak in a phosphorus-doped fiber to enable the cladding pump, the QD is reduced to as low as 0.78% with a 23.7 W output power. To our knowledge, this is the lowest QD ever reported in a cladding-pumped RFL. Furthermore, the output power can be scaled to 47.7 W with a QD of 1.29%. This work not only offers a preliminary platform for the realization of high-power low-QD fiber lasers, but also proves the great potential of low-QD fiber lasers in power scaling.

Using the example of the PHELIX high-energy short pulse laser we discuss the technical preconditions to investigate ion acceleration with submicrometer thick targets. We show how the temporal contrast of this system was improved to prevent pre-ionization of such targets on the nanosecond timescale. Furthermore the influence of typical fluctuations or uncertainties of the on-target intensity on ion acceleration experiments is discussed. We report how these uncertainties were reduced by improving the assessment and control of the on-shot intensity and by optimizing the positioning of the target into the focal plane. Finally we report on experimental results showing maximum proton energies in excess of 85 MeV for ion acceleration via the target normal sheath acceleration mechanism using target thicknesses on the order of one micrometer.

After a population of laser-driven hot electrons traverses a limited thickness solid target, these electrons will encounter the rear surface, creating TV/m fields that heavily influence the subsequent hot-electron propagation. Electrons that fail to overcome the electrostatic potential reflux back into the target. Those electrons that do overcome the field will escape the target. Here, using the particle-in-cell (PIC) code EPOCH and particle tracking of a large population of macro-particles, we investigate the refluxing and escaping electron populations, as well as the magnitude, spatial and temporal evolution of the rear surface electrostatic fields. The temperature of both the escaping and refluxing electrons is reduced by 30%–50% when compared to the initial hot-electron temperature as a function of intensity between $10^{19}$ and $10^{21}~~\text{W}/\text{cm}^{2}$. Using particle tracking we conclude that the highest energy internal hot electrons are guaranteed to escape up to a threshold energy, below which only a small fraction are able to escape the target. We also examine the temporal characteristic of energy changes of the refluxing and escaping electrons and show that the majority of the energy change is as a result of the temporally evolving electric field that forms on the rear surface.

We demonstrate a monolithic single frequency Tm-doped fiber amplifier with output power of 51.5 W. A single frequency fiber laser at 1.97 $\mathrm {\mu} $m is amplified by a cascaded master oscillator power amplifier (MOPA) system with all-fiber configuration. The optical-to-optical conversion efficiency of the main fiber amplifier is 45%. No amplified spontaneous emission (ASE) or stimulated Brillouin scattering (SBS) effect is observed in the fiber amplifier. The output power could be further scaled by launching more pump power.